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Chemistry of Aerosols over Chukchi Sea and Bering Sea

朱赖民 陈立奇 杨绪林 杜俊民 张远辉

中国地球化学学报(英文版)2004,Vol.23Issue(1):26-36,11.
中国地球化学学报(英文版)2004,Vol.23Issue(1):26-36,11.

Chemistry of Aerosols over Chukchi Sea and Bering Sea

Chemistry of Aerosols over Chukchi Sea and Bering Sea

朱赖民 1陈立奇 1杨绪林 1杜俊民 1张远辉1

作者信息

  • 1. The Third Institute of Oceanography, Key Laboratory of Global Change and Marine-Atmospheric Chemistry, SOA, Xiamen 361005, China
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摘要

Abstract

The contents of elements in aerosols sampled during the First Chinese Arctic Research Expedition (CHINARE-1) show great differences from one element to another. Na, K,Ca, Mg, Al, F, and Cl are the major components in the aerosols, whose contents are larger than 30 ng/m3. The chemical elements whose contents vary between 0.1-30 ng/m3 are Br,Sr, Cr, Ni, and Zn. The chemical elements whose contents are close to or slightly higher than 0. 1 ng/m3 are Rb, Ba, Zr, Th, and Pb. The contents of As, Sb, W, Mo, Au, La, Ce, Nd,Sm, Eu, Tb, Yb, Lu, Sc, Co, Hf, Ta, and Cd are less than 0.1 ng/m3. The mass concentration data for the same element, as observed during CHINARE-1, are almost accordant, but much lower than what is observed in the China' s seas or the coasts of China. The enrichment factor and electron microscopic analyses and lead isotope tracing were used to distinguish their sources.Four groups of sources can be classified as follows: anthropogenic: As, Sb, W, F, Mo, Au,Cu, Pb, Cd, V; crustal: La, Ce, Nd, Sm, Eu, Tb, Yb, Lu, Fe, Sc, Cr, Co, Ba, Zr, Hf,Ta, Cs, Mn, Th, U; oceanic:Na, K, Ca, and Mg; and mixing: Rb, Sr, Ca, and Mg.

关键词

marine aerosol/global change/Arctic/CHINARE-1

Key words

marine aerosol/global change/Arctic/CHINARE-1

分类

天文与地球科学

引用本文复制引用

朱赖民,陈立奇,杨绪林,杜俊民,张远辉..Chemistry of Aerosols over Chukchi Sea and Bering Sea[J].中国地球化学学报(英文版),2004,23(1):26-36,11.

基金项目

This research project was granted jointly by the National Natural Science Foundation of China (Grant No. 40006005), the First Arctic Research Expedition Program, and the key projects supported by the Youth Foundation sponsored by the State Ocean Adminis-t (Grant No. 40006005)

中国地球化学学报(英文版)

2096-0956

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