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光激发下分子纳米结中电荷输运的振动效应研究

李金花 王鹿霞

物理学报2011,Vol.60Issue(11):632-638,7.
物理学报2011,Vol.60Issue(11):632-638,7.

光激发下分子纳米结中电荷输运的振动效应研究

Vibrational effect on external field control of charge transmission in molecular nano-junction

李金花 1王鹿霞1

作者信息

  • 1. 北京科技大学数理学院物理系,北京100083
  • 折叠

摘要

Abstract

With the weak-coupling approach in molecular vibrational normal coordinate,the charge transmission under external optical field through molecular nano-junction is studied.From the charging energy point of view,the sequential charge transmission is analyzed and the current-voltage characteristics under external optical field are studied.It is found that the vibrational effect of molecule is the key factor of the removal of Franck-Condon blockage under external optical field.Furthermore,the effects of charging energy and intra-molecular vibrational energy redistribution (IVR) in charge transmission under external optical field are studied in detail.

关键词

Franck-Condon阻滞/振动效应/电流-电压特性

Key words

Franck-Condon blockage/vibrational effect/current-voltage characteristics

分类

数理科学

引用本文复制引用

李金花,王鹿霞..光激发下分子纳米结中电荷输运的振动效应研究[J].物理学报,2011,60(11):632-638,7.

基金项目

中央高校基本科研业务费专项资金 ()

国家自然科学基金(批准号:11174029)资助的课题 ()

物理学报

OA北大核心CSCDCSTPCDSCI

1000-3290

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