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脉冲激光烧蚀制备纳米Si晶粒成核气压阈值及动力学研究

邓泽超 罗青山 丁学成 褚立志 梁伟华 陈金忠 傅广生 王英龙

物理学报2011,Vol.60Issue(12):433-437,5.
物理学报2011,Vol.60Issue(12):433-437,5.

脉冲激光烧蚀制备纳米Si晶粒成核气压阈值及动力学研究

Pressure threshold and dynamics of nucleation for Si nano-crystal grains prepared by pulsed laser ablation

邓泽超 1罗青山 1丁学成 1褚立志 1梁伟华 1陈金忠 1傅广生 1王英龙1

作者信息

  • 1. 河北大学物理科学与技术学院,河北省光电信息材料重点实验室,保定071002
  • 折叠

摘要

Abstract

Si nano-crystal grains are prepared by pulsed laser ablation in low pressure Ar at room temperature through changing the gas pressure and the distance between target and substrate.The morphologies and compositions of samples are characterized by scanning electron microscopy images,Raman scattering spectra and X-ray diffraction spectra.The pressure threshold for Si grain formation is obtained to be 0.6 Pa at a laser fluence of 4 J/cm2,distance between target and substarate of 3 cm,and room temperature.Combining the fluid mechanics model and the nucleation division model,the dynamics process of nucleation is analyzed.The Monte Carlo simulation shows that the nucleation of nano-crystal grains is determined jointly by temperature and supersaturated density.

关键词

脉冲激光烧蚀/成核/气压阈值/Monte/Carlo数值模拟

Key words

pulsed laser ablation/nucleation/pressure threshold/Monte Carlo simulation

分类

数理科学

引用本文复制引用

邓泽超,罗青山,丁学成,褚立志,梁伟华,陈金忠,傅广生,王英龙..脉冲激光烧蚀制备纳米Si晶粒成核气压阈值及动力学研究[J].物理学报,2011,60(12):433-437,5.

基金项目

国家重点基础研究发展计划前期专项基金 ()

国家自然科学基金 ()

河北省自然科学基金 ()

河北省教育厅科研基金(批准号:2009308)资助的课题 ()

物理学报

OA北大核心CSCDCSTPCDSCI

1000-3290

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