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TiO2/石墨烯纳米复合材料制备及其光催化性能研究

周建伟 王储备 禇亮亮 张明瑛 史磊

人工晶体学报2013,Vol.42Issue(4):762-767,6.
人工晶体学报2013,Vol.42Issue(4):762-767,6.

TiO2/石墨烯纳米复合材料制备及其光催化性能研究

Preparation and Photocatalytic Performance of TiO2/Graphene Nano-composite Material

周建伟 1王储备 1禇亮亮 1张明瑛 1史磊1

作者信息

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摘要

Abstract

TiO2/graphene composite photocatalyst has been prepared by a facile liquid phase deposition method using titanium trifluoride and graphene oxide as the raw materials.The products were characterized by X-ray diffraction, scanning electron microscopy, X-ray photoelectron spectroscopy and UV-Visible analysis.It was found that the reduction graphene was covered with petal-like anatase TiO2 nanoparticles, which were more uniform and smaller in size.The photocatalytic activities were evaluated using the photocatalytic reduction of CO2.Photocatalytic reduction of CO2 with H2O in the aqueous phase is studied by using TiO2/graphene catalyst under UV irradiation.The results showed that the compostie exhibited significantly photocatalytic reduction activities and reaction products high selectivity, reaction 6 h methanol accumulated production for 3.43 mmol/L.Graphene effectively improved the photocatalytic activity and reaction efficiency of the semiconductor, and synergistic effect was obvious.

关键词

TiO2/石墨烯复合材料/光催化/协同效应/反应机理

Key words

TiO2/graphene composites/ photocatalysis/ synergistic effect/ reaction mechanism

分类

化学化工

引用本文复制引用

周建伟,王储备,禇亮亮,张明瑛,史磊..TiO2/石墨烯纳米复合材料制备及其光催化性能研究[J].人工晶体学报,2013,42(4):762-767,6.

基金项目

河南省高校科技创新人才支持计划项目资助(2010HASTTT040) (2010HASTTT040)

人工晶体学报

OA北大核心CSCDCSTPCD

1000-985X

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