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氧化物催化剂对非热等离子体催化降解甲苯的影响

张玮 杨懿 王沛涛 吴军良 付名利 黄碧纯 叶代启

环境工程学报2013,Vol.7Issue(7):2655-2661,7.
环境工程学报2013,Vol.7Issue(7):2655-2661,7.

氧化物催化剂对非热等离子体催化降解甲苯的影响

Impact of oxide catalysts on toluene destruction by non-thermal plasma

张玮 1杨懿 1王沛涛 1吴军良 1付名利 2黄碧纯 1叶代启2

作者信息

  • 1. 华南理工大学环境与能源学院,广州510006
  • 2. 广东省大气环境与污染控制重点实验室,广州510006
  • 折叠

摘要

Abstract

The effects of different oxide catalysts on NTP catalytic decomposition toluene in dry atmosphere were investigated in this work.For different catalysts,the decomposition efficiency of toluene,carbon balance,CO2 selectivity and O3 removal were studied through the dielectric property,surface oxygen delivery capacity,specific surface area and pore structure,respectively.The results show that the decomposition efficiency of toluene,carbon balance and the outlet concentration of O3 can be improved by the dielectric property.However,the dielectric property doesn' t affect the CO2 selectivity and O3 removal at all.For a given specific energy density,the effect of specific surface area and pore structure on the CO2 selectivity and O3 removal is more significant than dielectric property.Additionally,the surface oxygen delivery capacity of the catalysts could promote obviously the decomposition reaction of toluene,and the influence is stronger than specific surface area and pore structure.

关键词

氧化物/催化剂/非热等离子体/甲苯/表面供氧能力

Key words

oxide / catalyst / non-thermal plasma / toluene / surface oxygen delivery capacity

分类

资源环境

引用本文复制引用

张玮,杨懿,王沛涛,吴军良,付名利,黄碧纯,叶代启..氧化物催化剂对非热等离子体催化降解甲苯的影响[J].环境工程学报,2013,7(7):2655-2661,7.

基金项目

国家"863"高技术研究发展计划项目(2013AA065005) (2013AA065005)

国家自然科学基金资助项目(50978103,51108187) (50978103,51108187)

中央高校基金科研业务费专项资金项目(2012ZM0041) (2012ZM0041)

环境工程学报

OA北大核心CSCDCSTPCD

1673-9108

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