化工进展Issue(6):1652-1655,4.DOI:10.16085/j.issn.1000-6613.2015.06.025
Mn、Ce负载顺序对催化剂Mn-Ce/TiO2低温脱硝活性的影响
Effect of loading sequence of Mn and Ce on the activity of Mn-Ce/TiO2 catalysts at low-temperature
摘要
Abstract
Manganese and cerium oxide catalysts were prepared by sol-gel method and used for the low-temperature selective catalytic reduction (SCR) of NO with NH3. The catalysts were characterized by BET surface area,X-ray diffraction (XRD) and scanning electron microscope (SEM). The influence of loading sequence on the structure of Mn-Ce/TiO2 catalysts was investigated. The results showed that the phase structure of catalysts was anatase. Mn and Ce distributed in amorphous form. When Mn and Ce were supported on same carrier,the specific surface area of catalyst was the largest,which achieved 97.6m2/g,and active components of Mn and Ce were well distributed. The catalyst activity was also the highest when Mn and Ce were supported on same carrier. The NO removal efficiency was above 90%, when the reaction temperature was 200℃.关键词
催化剂/选择催化还原/活性/负载顺序/烟气脱硝Key words
catalyst/selective catalytic reduction (SCR)/reactivity/loading sequence/flue gas denitration分类
资源环境引用本文复制引用
闫东杰,玉亚,徐颖,黄学敏..Mn、Ce负载顺序对催化剂Mn-Ce/TiO2低温脱硝活性的影响[J].化工进展,2015,(6):1652-1655,4.基金项目
陕西省教育厅科研计划(14JK1392)及西安建筑科技大学科技基金(DB03132、DA03124)项目。 ()