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中空纤维空气隙式膜蒸馏海水淡化过程的性能模拟与优化

李卜义 王建友 王济虎 刘红斌

化工学报Issue(2):118-125,8.
化工学报Issue(2):118-125,8.DOI:10.11949/j.issn.0438-1157.20141164

中空纤维空气隙式膜蒸馏海水淡化过程的性能模拟与优化

Modeling and optimization of hollow fiber air gap membrane distillation for seawater desalination

李卜义 1王建友 1王济虎 2刘红斌2

作者信息

  • 1. 南开大学环境科学与工程学院,天津 300071
  • 2. 军事医学科学院卫生装备研究所,天津 300161
  • 折叠

摘要

Abstract

Response surface methodology (RSM) was used for modeling and optimization of operating parameters and permeate flux for hollow fiber air gap membrane distillation (AGMD-HF) desalination process with simulated 3.5%(mass) seawater as feed solution. Hot feed-in temperature, cold feed-in temperature and fluid flow rate were chosen for experiment optimization based on central composite design (CCD). A quadratic polynomial regression model for permeate flux and operating parameters was developed. Accuracy of the model was validated by analysis of variance (ANOVA), RSM and comparison of predicted and experimental permeate flux response. Furthermore,the best optimal level of operating parameters and solar-powered verification were performed. During the experiments,permeate conductivity was constantly kept below 10μS·cm−1, and relative ion rejection rate was above 99.99%. A R2 of 0.986,p-value smaller than 0.0001 for ANOVA were obtained, and average error of predicted and experimental permeate flux was 6.95%. Moreover, the best optimal operating parameters of 83.5℃,13.2℃ and 60.2 L·h−1 based on desirability function and solar-powered process permeate flux of 6.47 L·m−2·h−1 were presented. Consequently, modeling and optimization of operating parameters for permeate flux response could be helpful for scaling up AGMD-HF desalination process, and introduction of solar power as an alternative of conventional electric heat source could have better application prospect for AGMD-HF desalination.

关键词

响应曲面/中空纤维空气隙式膜蒸馏/模拟/优化/蒸馏/脱盐/设计

Key words

response surface methodology/hollow fiber air gap membrane distillation/modeling/optimization/distillation/desalination/design

分类

化学化工

引用本文复制引用

李卜义,王建友,王济虎,刘红斌..中空纤维空气隙式膜蒸馏海水淡化过程的性能模拟与优化[J].化工学报,2015,(2):118-125,8.

基金项目

天津市科技兴海专项资金项目(KJXH2013-02)。 ()

化工学报

OA北大核心CSCDCSTPCD

0438-1157

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