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磁控溅射沉积铝/贫铀与金/贫铀镀层的界面研究*

易泰民 马坤全 邢丕峰 郑凤成 梅鲁生 杨蒙生 赵利平 李朝阳 谢军 杜凯

物理学报Issue(10):392-398,7.
物理学报Issue(10):392-398,7.DOI:10.7498/aps.62.108101

磁控溅射沉积铝/贫铀与金/贫铀镀层的界面研究*

Study on interface of Al/depleted uranium and Au/depleted uranium layers deposited by magnetron sputtering∗

易泰民 1马坤全 1邢丕峰 1郑凤成 1梅鲁生 1杨蒙生 1赵利平 1李朝阳 1谢军 1杜凯1

作者信息

  • 1. 中国工程物理研究院激光聚变研究中心,绵阳 621900
  • 折叠

摘要

Abstract

Aluminum/depleted uranium/aluminum (Al/DU/Al) and gold/depleted uranium/gold (Au/DU/Au)“sandwich structure”films are deposited by magnetron sputtering. Diffusions of Al/DU and Au/DU interface of these samples are investigated by high resolution scanning electronic microscope, X-ray diffraction, X-ray photoelectron spectrometer and scanning auger microprobe. The results show that deposited DU layer is of columnar grain. Significant diffusion takes place at Al/DU interface. Intermetallic compounds of Al2U and Al3U are formed at Al/DU interface by chemical reaction between Al and DU which induces chemical shift toward high binding energy of Al 2p and toward low binding energy of U 4f. Microdosages of O exist in Al over-layers as Al2O3, in Al/DU interface as Al2O3 and oxidation of uranium, and in DU layers as oxidation of uranium respectively. Just simple physical diffusion takes place at Au/DU interface. Binding energies of Au 4f and U 4f shift toward high-energy tail induced by cluster effect at the Au/DU interface. Microdosages of O exist at Au/DU interface and in DU layers as oxidation of uranium. Diffusion at the Al/DU interface is more obvious than at Au/DU surface. Under the condition of the same thickness valuses Al over-layer is more effective than Au over layer to protect uranium layer from oxidging.

关键词

Al/DU界面/Au/DU界面/磁控溅射/界面扩散

Key words

Al/DU interface/Au/DU interface/magnetron sputtering/diffusion at interface

引用本文复制引用

易泰民,马坤全,邢丕峰,郑凤成,梅鲁生,杨蒙生,赵利平,李朝阳,谢军,杜凯..磁控溅射沉积铝/贫铀与金/贫铀镀层的界面研究*[J].物理学报,2013,(10):392-398,7.

基金项目

国家重点基础研究发展计划(批准号:2011CB610402)和国家自然科学基金(批准号:50971102,50901061)资助的课题.@@@@Project supported by the National Basic Research Program of China (Grant No.2011CB610402), and the National Natural Science Foundation of China (Grant Nos.50971102,50901061) (批准号:2011CB610402)

物理学报

OA北大核心CSCDCSTPCD

1000-3290

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