化工进展2016，Vol.35Issue(7)：1929-1941,13.DOI:10.16085/j.issn.1000-6613.2016.07.001
大气压冷等离子体与水溶液作用过程的数值模拟研究进展
Research progress on numerical simulation of cold atmospheric plasmas on aqueous solutions
摘要
Abstract
As an effective and complex chemical reaction field,cold atmospheric plasma (CAP) has been extensively studied and applied in biotechnology,medical science,environmental protection, materials science,and so on. Since aqueous solution is usually used as the reaction media among numerous applications of the CAPs,the understandings of the interaction mechanism between the CAP and aqueous solution is of great importance. However,due to the big complexity of CAP-solution interaction processes,the present experimental methods are still quite difficult to comprehensively reveal the action mechanisms. Numerical simulation has thus been employed widely in the CAP field and become one of important methods to investigate the interaction mechanisms of CAP with solution. In this review,we focus on the simulation methods used for exploring the interaction mechanisms between the CAP and aqueous solution,including fluid dynamics modelling and molecular dynamics simulation. For the fluid dynamics modelling,this review gives a detailed description of the features of the global,one- and two-dimensional models and their applications in analysis of the interactions of the dielectric barrier discharge (DBD) and plasmas jets with aqueous solution. On the other hand,the interaction process between reactive oxygen species (ROS) and biomolecules in aqueous solution by employing the molecular dynamics simulation method based on reactive force field is also reviewed. The advantages and disadvantages of fluid dynamics modelling and molecular dynamics simulation are then compared,and a brief discussion on the urgent problems as well as the perspectives of the future development in this field has been also described.关键词
大气压冷等离子体/水溶液/流体力学模拟/分子动力学模拟/突变Key words
cold atmospheric pressure plasma/aqueous solution/fluid dynamics model/molecular dynamics simulation/mutation分类
化学工程引用本文复制引用
常海波,张雪,张晓菲,张翀,李和平,邢新会..大气压冷等离子体与水溶液作用过程的数值模拟研究进展[J].化工进展,2016,35(7):1929-1941,13.基金项目
清华大学自主科研计划（52300600516）、日本JST CREST项目及中国博士后基金（2014M550742）项目。 （）
