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碳纳米管/BiOBr复合材料可见光光催化脱色染料废水

许润铭 方群凯 朱翩翩 蒋茹 朱华跃

印染助剂2017,Vol.34Issue(2):7-11,5.
印染助剂2017,Vol.34Issue(2):7-11,5.

碳纳米管/BiOBr复合材料可见光光催化脱色染料废水

Photocatalytic decolorization of dye wastewater containing congo red with carbon nanotube/BiOBr composite photocatalyst

许润铭 1方群凯 1朱翩翩 1蒋茹 1朱华跃1

作者信息

  • 1. 台州学院环境工程系,浙江台州 318000
  • 折叠

摘要

Abstract

The composite photocatalyst carbon nanotube/BiOBr (MWCNTs/BiOBr) was prepared by hydro⁃thermal method using multi- wal ed carbon nanotubes (MWCNTs), KBr and Bi(NO3)3·5H2O as raw materials. The photocatalytic activity of the photocatalyst under xenon lamp was studied using congo red as the target pol utant. The effects of photocatalyst dosage, congo red initial concentration, anion species on the decoloriza⁃tion of congo red were investigated and the stability of photocatalyst was also verified. The results showed that the introduction of carbon nanotubes could make the photocatalytic activity and adsorption performance of the MWCNTs/BiOBr composite significantly better than BiOBr. The decolorization was as high as 99%when catalyst dosage was 1.5 g/L , the initial concentration of congo red was 15 mg/L, and the photocatalytic time was 120 min. The main active species in the reaction system were hole (h+) and hydroxide radical (·OH). The decolorization of congo red could stil reach more than 92%after 4 repeated cycle use.

关键词

BiOBr/碳纳米管/光催化/脱色/刚果红

Key words

BiOBr/carbon nanotube/photocatalytic/decolorization/congo red

分类

资源环境

引用本文复制引用

许润铭,方群凯,朱翩翩,蒋茹,朱华跃..碳纳米管/BiOBr复合材料可见光光催化脱色染料废水[J].印染助剂,2017,34(2):7-11,5.

基金项目

浙江省自然科学基金项目(LY14B070011,LY15E080002);国家自然科学基金项目(Grant No.51208331);国家大学生创新创业训练计划项目(201410350008);浙江省大学生科技创新项目 ()

印染助剂

OA北大核心CSTPCD

1004-0439

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