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用于二苯并噻吩高效催化氧化多酸基复合材料的制备

王红菊 赵吉祥 刘娜 翟尚儒

硅酸盐通报2017,Vol.36Issue(1):321-324,4.
硅酸盐通报2017,Vol.36Issue(1):321-324,4.

用于二苯并噻吩高效催化氧化多酸基复合材料的制备

Preparation of High-performance HPW-based Catalyst for Dibenzothiophene Oxidation

王红菊 1赵吉祥 2刘娜 2翟尚儒2

作者信息

  • 1. 呼伦贝尔学院化学与化工学院,呼伦贝尔 021008
  • 2. 大连工业大学轻工与化学工程学院,大连 116034
  • 折叠

摘要

Abstract

A layer-by-layer stabilization strategy was employed to immobilize active tungstophosphoric acid onto pentaethylenehexamine-preloaded ZrSBA-15. The synthesized materials were characterized by XRD, N2 adsorption-desorpton isotherms, FT-IR and TEM, etc. Utilizing hydrogen peroxide as oxidant, the composite exhibited favorable performance toward the deep oxidation desulfurization of dibenzothiophene;and it could be reused at least six runs without discernible decrease in activity.

关键词

氧化脱硫/多酸/催化/SBA-15

Key words

oxidization desulfurization/heteropolyacids/catalysis/SBA-15

分类

化学化工

引用本文复制引用

王红菊,赵吉祥,刘娜,翟尚儒..用于二苯并噻吩高效催化氧化多酸基复合材料的制备[J].硅酸盐通报,2017,36(1):321-324,4.

基金项目

国家自然科学基金(21676039) (21676039)

硅酸盐通报

OA北大核心CSCDCSTPCD

1001-1625

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