化工进展2017，Vol.36Issue(z1)：278-290,13.DOI:10.16085/j.issn.1000-6613.2017-0196
二氧化碳捕获固体吸附剂的研究进展
Research progress of solid adsorbent for CO2 capture
摘要
Abstract
Post-combustion CO2 capture is of paramount importance in CO2 capture and storage technology.As a common post-combustion method,solid adsorbents possess advantage of low energy consumption,low corrosion,and favorable regenerability as well as simple devices.It exerts great influence in the realization of CO2-reduction targets.The key of using adsorption method to eliminate the CO2 concentration is that the research&development of adsorbent with large adsorption capacity,high selectivity,and lower energy consumption.This paper focuses on recent research progress of carbon-based adsorbents,zeolites,metal-oxide,amino-adsorbents, and metal-organic frameworks (MOFs ).We mainly elaborate the physical and chemical properties and enumerate CO2 adsorption properties in practice, existing problems and the improvement measures of these adsorbents.Besides, this paper emphases on the application prospect of metal-organic frameworks in the flue gas.It is shown that MOFs are promising adsorbents due to its high specific area, large pore volume, high porosity, structure tunability.In order to improve the CO2 adsorption properties of MOFs, four modification methods are summarized in this paper.It extends idea for the worker who will engaged in research and development of CO2 adsorbents.关键词
二氧化碳/吸附剂/吸附(作用)/分离/烟道气Key words
carbon dioxide/adsorbents/adsorption/separation/flue gas分类
化学化工引用本文复制引用
辛春玲,王素青,孟庆国,刘丽丽,王霞,杨金美..二氧化碳捕获固体吸附剂的研究进展[J].化工进展,2017,36(z1):278-290,13.基金项目
潍坊市科技发展计划(2016GX013)、潍坊学院博士科研基金(2016BS09)及山东省自然科学基金(联合专项)(ZR2013BL016)项目. （2016GX013）
