物理化学学报2018，Vol.34Issue(4)：361-376,16.DOI:10.3866/PKU.WHXB201708312
维度调控策略提升铂基纳米晶氧还原催化研究进展
Boosting Oxygen Reduction Catalysis by Tuning the Dimensionality of Pt-based Nanostructures
摘要
Abstract
The past decade has witnessed tremendous progress in the improvement of the electrocatalytic efficiency of the oxygen reduction reaction (ORR),which is important for the widespread adoption of fuel cells.This review provides an overview of the recent advances in the rational structural design and construction of Pt-based nanocatalysts to achieve higher ORR activity,with an emphasis on tuning the dimensionalities of Pt-based nanocrystals.The advantages and disadvantages of each dimensional catalyst have been discussed.In particular,we focus on a contemporary understanding of the structure-performance relationships based on the combined theoretical and experimental evidence,which can be further applied to guide the search for more exciting catalytic systems.The review concludes with a personal perspective for future research directions.关键词
燃料电池/氧还原/铂基纳米晶/维度调控Key words
Fuel cells/Oxygen reduction reaction/Platinum-based nanocrystals/Dimensionality tuning分类
化学化工引用本文复制引用
骆明川,孙英俊,秦英楠,杨勇,吴冬,郭少军..维度调控策略提升铂基纳米晶氧还原催化研究进展[J].物理化学学报,2018,34(4):361-376,16.基金项目
The project was supported by the National Natural Science Foundation of China (51671003),the China Postdoctoral Science Foundation (2017M610022),the National Basic Research Program of China (2016YFB0100201),the Open Project Foundation of State Key Laboratory of Chemical Resource Engineering,the start-up supports from Peking University,and the Young Thousand Talented Program,China.国家自然科学基金(51671003),博士后基金(2017M610022),国家重点基础研究发展计划(2016YFB0100201),资源有效利用国家重点实验室开放项目,北京大学启动项目和千人计划青年项目资助 （51671003）
