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钕负载二氧化钛-炭杂化气凝胶的制备及其光催化性能

邵霞 潘峰 郑励 张睿 张文雅

新型炭材料2018,Vol.33Issue(2):116-124,9.
新型炭材料2018,Vol.33Issue(2):116-124,9.DOI:10.1016/S1872-5805(18)60329-4

钕负载二氧化钛-炭杂化气凝胶的制备及其光催化性能

Nd-doped TiO2-C hybrid aerogels and their photocatalytic properties

邵霞 1潘峰 2郑励 1张睿 1张文雅1

作者信息

  • 1. 上海应用技术大学,材料科学与工程学院,上海201418
  • 2. 上海应用技术大学,化学与环境工程学院,上海201418
  • 折叠

摘要

Abstract

Nd-doped TiO2-C hybrid aerogels with different Nd doping levels were prepared by a combined sol-gel and impregna-tion method. The microstructure,morphology and photocatalytic activities of the samples were investigated by XRD,SEM,FTIR, XPS, nitrogen adsorption and the photocatalytic degradation of methylene blue(MB) under UV irradiation. Results showed that the samples are composed of irregular-shaped nanoparticles and the Nd dopant inhibits their growth. The TiO2in the samples is anatase, the carbon is amorphous and Nd3+is in a Ti-O-Nd bond form. The samples had strong absorption in the ultraviolet region and exhibi-ted good degradation activity for MB in aqueous solutions under UV light. The best activity was achieved when the ratio of Nd to Ti is 3-4 wt%,in which case MB was completely degraded under UV irradiation for 160 min.

关键词

光催化性/降解/钕负载/亚甲基蓝/溶胶凝胶法

Key words

Photo-catalysts/Degradation/Nd-doped/MB/Sol-gel method

分类

通用工业技术

引用本文复制引用

邵霞,潘峰,郑励,张睿,张文雅..钕负载二氧化钛-炭杂化气凝胶的制备及其光催化性能[J].新型炭材料,2018,33(2):116-124,9.

基金项目

上海地方高校能力建设项目(12160503600) (12160503600)

上海市一流学科建设项目(J201212) (J201212)

国家自然科学基金项目(U1332107) (U1332107)

上海应用技术大学复合材料重点学科建设项目(10210Q140001).Capacity Building Program of Shanghai Local Universities(12160503600) (10210Q140001)

The First-Class Discipline Construction Fund of Shanghai Municipal Education Commission(J201212) (J201212)

Natinal Natural Science Foundation of China(U1332107) (U1332107)

Key Discipline Construction Fund of Composite Materials of Shanghai Institute of Technology(10210Q140001). (10210Q140001)

新型炭材料

OA北大核心CSCDCSTPCDSCI

1007-8827

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