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钠添加剂对介质阻挡-电晕放电耦合法尿素脱除NO的影响

李艳荣 张香 杨岚 贺建勋 闵小建 樊英杰 马晓迅

化工进展2018,Vol.37Issue(5):1978-1984,7.
化工进展2018,Vol.37Issue(5):1978-1984,7.DOI:10.16085/j.issn.1000-6613.2017-1365

钠添加剂对介质阻挡-电晕放电耦合法尿素脱除NO的影响

Effects of sodium additives on NO removal of urea by dielectric barrier -corona discharge coupling method

李艳荣 1张香 1杨岚 1贺建勋 1闵小建 1樊英杰 1马晓迅1

作者信息

  • 1. 西北大学化工学院,国家碳氢资源清洁利用国际科技合作基地,陕北能源先进化工利用技术教育部工程研究中心,陕西省洁净煤转化工程技术研究中心,陕北能源化工产业发展协同创新中心,陕西煤业化工技术研究院有限责任公司,陕西 西安 710069
  • 折叠

摘要

Abstract

The effects of different sodium additives(Na2CO3、NaOH、CH3COONa)on the removal of the NO by urea and the mechanism of the NO removal were investigated on a self-designed dielectric barrier-corona discharge coupling device. The results indicated that,within the scope of the study,the NO removal rate increased with the increase of the urea content. The NO removal rate was 64.23% with 0.3% urea added at 0.83A current. However,the CO was produced and increased with the increasing of the dosage of urea;the addition of a small amount of sodium additives could significantly improve the NO removal rate that increased with the increase of the content of sodium additives. The amount of CO production was effectively inhibited. Under the same dosages,various sodium additives could promote the NO removal of urea. The NO removal was affected by the sodium additive in accordance with the order of NaOH>Na2CO3>CH3COONa. NO removal rate was 90.71% and 95.71% at 0.83A and 5A current,respectively;when sodium hydroxide and urea mass ratio was 10:10.while there was almost no CO.

关键词

介质阻挡-电晕放电耦合法/一氧化氮/脱除率/尿素/添加剂

Key words

dielectric barrier and corona discharge/nitric oxide/removal efficiency/urea/additive

分类

资源环境

引用本文复制引用

李艳荣,张香,杨岚,贺建勋,闵小建,樊英杰,马晓迅..钠添加剂对介质阻挡-电晕放电耦合法尿素脱除NO的影响[J].化工进展,2018,37(5):1978-1984,7.

基金项目

国家自然科学基金(21536009)及陕西省科技计划(2017ZDCXL-GY-10-03)项目. (21536009)

化工进展

OA北大核心CSCDCSTPCD

1000-6613

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