太原理工大学学报2018,Vol.49Issue(3):386-390,5.DOI:10.16355/j.cnki.issn1007-9432tyut.2018.03.003
新型Mn-Fe/ZSM-5催化剂的NH3-SCR脱硝性能
De-NOxPerformance of Novel Mn-Fe/ZSM-5 Catalysts for NH3-SCR
摘要
Abstract
Mn-Fe/ZSM-5 catalyst was prepared by ammonia precipitation-chemical vapor dep-osition method and its performance of the selective catalytic reduction of NO by NH3(NH3-SCR) was investigated.Mn-Fe/ZSM-5 catalyst had better low temperature SCR activity and wider ac-tivity temperature range.NO conversion on it was up to 98% at 180~450 ℃.Meanwhile,this catalyst had better dispersity,higher ability of redox,more appropriate acidity and better resist-ance to SO2.The active components Mn and Fe over Mn-Fe/ZSM-5 catalyst had a synergetic in-teraction.In presence of SO2,Mn-Fe/ZSM-5 catalyst exhibited an excellent resisitance to SO2 with a NO conversion of above 98% at 240~450 ℃.关键词
NOx/NH3-SCR/氨水沉淀-化学蒸气沉积法/Mn-Fe/ZSM-5催化剂/活性Key words
NOx/NH3-SCR/ammonia precipitation-chemical vapor deposition method/Mn-Fe/ZSM-5 catalyst/activity分类
化学化工引用本文复制引用
苏丽清,邹春雷,冯雅琳,何凯,吴旭,李哲..新型Mn-Fe/ZSM-5催化剂的NH3-SCR脱硝性能[J].太原理工大学学报,2018,49(3):386-390,5.基金项目
国家自然科学基金资助项目(21336006) (21336006)
山西省科技攻关资助项目(20140313002-2) (20140313002-2)
山西省自然科学基金资助项目(201601D102007) (201601D102007)