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微型鼓泡器中甲烷水合物的生成特性

申小冬 任俊杰 梁德青

石油化工2018,Vol.47Issue(5):431-436,6.
石油化工2018,Vol.47Issue(5):431-436,6.DOI:10.3969/j.issn.1000-8144.2018.05.006

微型鼓泡器中甲烷水合物的生成特性

Formation characteristics of methane hydrate in a micro-bubbler

申小冬 1任俊杰 2梁德青3

作者信息

  • 1. 中国科学院 广州能源研究所 天然气水合物重点实验室 广州天然气水合物中心,广东 广州 510640
  • 2. 广东省新能源和可再生能源研究开发与应用重点实验室,广东 广州 510640
  • 3. 中国科学院大学,北京 100049
  • 折叠

摘要

Abstract

Effects of gas flow rates,pressures,temperatures and filter meshes in a high pressure bubbler on the formation kinetics and forms of methane gas hydrate in pure aquatic system are investigated. According to the experiment results,increasing the gas flow rate and pressure and decreasing the temperature can enhance methane hydrate formation rates. However,with the increase of the gas flow rate,gas conversion is reduced. Adding filter meshes may obviously enhance the hydrate formation rate and gas conversion and an optimum specification of filter mesh is 200. Such results also indicate that,it's very easy for methane hydrate to produce on the gas-liquid interface to result in formation of hydrate bubbles,and that the gas flow rate imposes a remarkable impact on the hydrate forms. When the gas flow rates is low,hydrate bubbles can keep their shape and are not easy to break,and they gather together with a loose texture,and conversely,gas is easy to escape when the gas flow rate is enhanced,and hydrate bubbles are easy to deform and break and aggregate with a relatively compact texture. Pressures and temperatures impose little effects on hydrate forms. Adding filter meshes can obviously decrease the gas bubble volume and more hydrate bubbles are formed.

关键词

鼓泡/甲烷/水合物/动力学/生成特性

Key words

bubbling/methane/hydrate/kinetics/formation characteristics

分类

能源科技

引用本文复制引用

申小冬,任俊杰,梁德青..微型鼓泡器中甲烷水合物的生成特性[J].石油化工,2018,47(5):431-436,6.

基金项目

国家自然科学基金项目(51376182). (51376182)

石油化工

OA北大核心CSCDCSTPCD

1000-8144

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