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改性拜耳法赤泥颗粒的制备及对土壤铅的稳定化处理

杨慧珠 程乾坤 王新璋 陈惠康 张红云 黄雄飞 杨晓芳 汤叶涛 石太宏

环境工程学报2018,Vol.12Issue(4):1171-1181,11.
环境工程学报2018,Vol.12Issue(4):1171-1181,11.DOI:10.12030/j.cjee.201710029

改性拜耳法赤泥颗粒的制备及对土壤铅的稳定化处理

Preparation of modified Bayer process red mud granules and stabilization treatment of lead in soil

杨慧珠 1程乾坤 1王新璋 2陈惠康 2张红云 1黄雄飞 1杨晓芳 3汤叶涛 2石太宏1

作者信息

  • 1. 中山大学环境科学与工程学院,广州510006
  • 2. 中电投山西铝业有限公司,原平034100
  • 3. 广东省环境污染控制与修复技术重点实验室,广州510006
  • 折叠

摘要

Abstract

A large amount of Bayer process red mud is produced every years.It is difficult to handle due to its complicate composition and alkalinity,causing environment pollution.Soil heavy metal pollution is grim in recent years,leading to child blood lead poisoning.Regarding the issue above,we prepared red mud granules by using the Bayer process red mud as the main raw material,adding a little cement and other modified additives,followed by the applicationin stabilizing the soil lead.The results indicated that the optimized parameters for the modification are materials of 2% cement + 5% gypsum + 5% fly ash + 5% calcium dihydrogen phosphate + 83% red mud,water cement ratio of 0.5,the disc granulation parameter of 28° < α < 40°and 20 r·min-1 < R < 40 r·min-1.The red mud particles prepared according to the optimized parameters are used to repair simulated soil with lead pollution at four different concentration which are 100,250,500 and 800 mg·kg-1.When dosing 5% red mud particles followed by 10 days' immobilization,the bioavailability of lead was reduced 72.52%、65.38%、64.73% and 40.03%,while the residual state increased by 43.4%,35.13%,43.42% and 43.97%,respectively.The residual state of soil lead has a tendency to increase as the pollution concentration of soil increase,indicating that red mud prepared into a granular material can effectively stabilize the different concentrations of lead in the soil.

关键词

赤泥/颗粒/土壤铅/稳定化

Key words

red mud/granules/Pb in soil/stabilization

分类

资源环境

引用本文复制引用

杨慧珠,程乾坤,王新璋,陈惠康,张红云,黄雄飞,杨晓芳,汤叶涛,石太宏..改性拜耳法赤泥颗粒的制备及对土壤铅的稳定化处理[J].环境工程学报,2018,12(4):1171-1181,11.

基金项目

广东省科技开发协作项目(71010623) (71010623)

环境工程学报

OA北大核心CSCDCSTPCD

1673-9108

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