新型炭材料2021，Vol.36Issue(3)：468-496,29.DOI:10.1016/S1872-5805(21)60034-3
多孔金属有机框架材料在甲烷存储与捕集中的研究进展及挑战
Porous metal–organic frameworks for methane storage and capture:status and challenges
摘要
Abstract
In the process of global transition to a sustainable low-carbon economy, the two major low-carbon energy technolo-gies, namely, methane (CH4) storage and methane capture face the same challenge, that is, the lack of efficient adsorbents. Metal-or-ganic framework (MOF) materials have potential value in the field of gas adsorption storage because of their high specific surface area, good porosity, and adjustable pore structure. In this study, the structural design and synthesis methods of MOFs are introduced, and the research progress and problems associated with MOF materials in methane storage and capture are reviewed. The current re-search status of methane storage at high pressure is introduced in terms of volumetric and gravimetric uptake. For methane capture at atmospheric pressure, emphasis is placed on CH4/N2 and CO2/CH4 separation and methane capture technologies. Finally, the prob-lems and challenges of using MOF materials to achieve efficient methane storage and capture are analyzed and future prospects are presented.关键词
金属有机框架/甲烷/吸附/储存/捕集Key words
Metal-organic frameworks/Methane/Adsorption/Storage/Capture分类
化学化工引用本文复制引用
李东泽,陈雷,刘刚,袁子云,李秉繁,张旭,魏甲强..多孔金属有机框架材料在甲烷存储与捕集中的研究进展及挑战[J].新型炭材料,2021,36(3):468-496,29.基金项目
This research was funded by the National Natur-al Science Foundation of China(51774315,51704319),the Fundamental Research Funds for the Central Uni-versities(18CX02172A). 国家自然科学基金项目(51774315,51704319),中央高校基本科研业务费专项资金(18CX02172A). （51774315,51704319）
