燃料化学学报2022,Vol.50Issue(2):243-249,7.DOI:10.1016/S1872-5813(21)60166-4
NiO改性C3N5光催化剂析氢性能研究
Nickel oxide modified C3N5 photocatalyst for enhanced hydrogen evolution performance
摘要
Abstract
Recently, a new carbon nitride (C3N5) photocatalyst has attracted much attention due to its excellent light harvesting and unique 2D structure. However, high recombination rates of electron-hole pairs of bulk C3N5 serious affect the photocatalytic performance. Herein, nickel oxide (NiO) modified C3N5 p-n junctions photocatalyst was synthesized by a facile hydrothermal method. Results indicated that the 9-Ni/C3N5 nanosheet photocatalyst showed excellent hydrogen production efficiency under visible light. The hydrogen production rate reached 357μmol/(g?h), which was 107-fold higher than that of pristine C3N5. The high catalytic performace was attributed to the 9-Ni/C3N5 p-n junctions which could efficiently promote photogenerated electron-hole pair separation and thus promote the hydrogen evolution reaction.关键词
制氢/C3N5纳米片/NiO/光催化Key words
hydrogenevolution/C3N5nanosheet/nickeloxide/photocatalysis分类
化学化工引用本文复制引用
刘慕瑶,王建云,段炼,刘宪,张磊..NiO改性C3N5光催化剂析氢性能研究[J].燃料化学学报,2022,50(2):243-249,7.基金项目
The project was supported by the Teaching Reform and Innovation Program of Higher Education Institutions in Shanxi(2020061)and the Teaching Reform and Innovation Program of Taiyuan University of Technology(2019013). (2020061)