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NiO改性C3N5光催化剂析氢性能研究

刘慕瑶 王建云 段炼 刘宪 张磊

燃料化学学报2022,Vol.50Issue(2):243-249,7.
燃料化学学报2022,Vol.50Issue(2):243-249,7.DOI:10.1016/S1872-5813(21)60166-4

NiO改性C3N5光催化剂析氢性能研究

Nickel oxide modified C3N5 photocatalyst for enhanced hydrogen evolution performance

刘慕瑶 1王建云 1段炼 1刘宪 2张磊3

作者信息

  • 1. 太原理工大学,化学化工学院,山西太原030024
  • 2. 太原师范学院,化学系,山西晋中030619
  • 3. 深圳华测国际认证有限公司,广东深圳518101
  • 折叠

摘要

Abstract

Recently, a new carbon nitride (C3N5) photocatalyst has attracted much attention due to its excellent light harvesting and unique 2D structure. However, high recombination rates of electron-hole pairs of bulk C3N5 serious affect the photocatalytic performance. Herein, nickel oxide (NiO) modified C3N5 p-n junctions photocatalyst was synthesized by a facile hydrothermal method. Results indicated that the 9-Ni/C3N5 nanosheet photocatalyst showed excellent hydrogen production efficiency under visible light. The hydrogen production rate reached 357μmol/(g?h), which was 107-fold higher than that of pristine C3N5. The high catalytic performace was attributed to the 9-Ni/C3N5 p-n junctions which could efficiently promote photogenerated electron-hole pair separation and thus promote the hydrogen evolution reaction.

关键词

制氢/C3N5纳米片/NiO/光催化

Key words

hydrogenevolution/C3N5nanosheet/nickeloxide/photocatalysis

分类

化学化工

引用本文复制引用

刘慕瑶,王建云,段炼,刘宪,张磊..NiO改性C3N5光催化剂析氢性能研究[J].燃料化学学报,2022,50(2):243-249,7.

基金项目

The project was supported by the Teaching Reform and Innovation Program of Higher Education Institutions in Shanxi(2020061)and the Teaching Reform and Innovation Program of Taiyuan University of Technology(2019013). (2020061)

燃料化学学报

OA北大核心CSCDCSTPCD

2097-213X

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