新型炭材料(中英文)2023,Vol.38Issue(4):659-677,19.DOI:10.1016/S1872-5805(23)60767-X
MXene基纳米材料在高性能金属锂负极应用中的研究进展
Recent advances in Mxene-based nanomaterials as hosts for high-performance lithium metal anodes and as additives for improving the properties of solid electrolytes
摘要
Abstract
To tackle the issues of rapid electrode degradation and severe safety issues caused by the uncontrollable growth of lith-ium dendrites in Li metal anodes(LMAs),two-dimensional transition metal carbides/nitrides(MXenes)with a high electrical con-ductivity,excellent mechanical properties,and abundant surface functional groups have been used as hosts to induce uniform Li nuc-leation and alleviate the volume changes,eventually inhibiting the formation of Li dendrites.Recent advances in the use of MXene-based nanomaterials in LMAs are summarized.The problems with using LMAs are first considered,and the ways of using MXene-based nanomaterials for suppressing Li dendrite growth and constructing stable LMAs are then summarized.These include the use of MXenes,MXene-metal hybrids,MXene-carbon hybrids,and MXene derivatives as hosts for the anodes and as additives to modify the electrolyte compositions to increase ionic conductivity and inhibit polymer crystallization.Finally,the challenges and prospects for using MXene-based nanomaterials in next-generation LMAs are briefly discussed.关键词
锂金属负极/MXene/枝晶/锂金属电池Key words
Lithium metal anodes/MXene/Dendrites/Lithium metal batteries分类
化学化工引用本文复制引用
杨佳璐,钱越,王可,袁华栋,佴建威,刘育京,王垚,罗剑敏,陶新永..MXene基纳米材料在高性能金属锂负极应用中的研究进展[J].新型炭材料(中英文),2023,38(4):659-677,19.基金项目
The authors acknowledge financial support by the National Natural Science Foundation of China(52225208,U21A20174,51972285 and 52202314). (52225208,U21A20174,51972285 and 52202314)