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Cr2O3中反铁磁自旋波的低频拉曼光谱研究

董彪 崔骏 田远哲 吴镝 张琦

物理学进展2023,Vol.43Issue(5):142-150,9.
物理学进展2023,Vol.43Issue(5):142-150,9.DOI:10.13725/j.cnki.pip.2023.05.002

Cr2O3中反铁磁自旋波的低频拉曼光谱研究

Low-Frequency Raman Detection of Antiferromagnetic Spin Waves in Cr2O3

董彪 1崔骏 1田远哲 1吴镝 1张琦1

作者信息

  • 1. 南京大学物理学院,固体微结构物理国家重点实验室,南京 210093
  • 折叠

摘要

Abstract

The antiferromagnetic(AFM)spin waves are promising for being utilized in high-speed and energy-efficient information processing.However,the excitation and detection of terahertz spin waves in AFM systems is challenging.Here,we demonstrate low-frequency Raman spectroscopy as a powerful tool for spin-wave detection in AFM systems.We present a systematic study of AFM magnons in Cr2O3,a prototypical uniaxial antiferromagnet,via Raman measurements down to 2.3 cm-1(69 GHz).We resolved the magnon Zeeman splitting and the spin-flop transition.We further determined the sign of angular momentum of the magnon branches via polarization-resolved Raman processes.We also obtained the anisotropy energy,the g-factor,and the spin-flop field of Cr2O3 as a function of temperatures and magnetic fields.A spin-wave renormalization theory accounts for all experimental observations.

关键词

反铁磁性/自旋波/低频拉曼光谱/自旋翻转

Key words

antiferromagnetism/spin wave/low-frequency Raman spectroscopy/spin-flop

分类

物理学

引用本文复制引用

董彪,崔骏,田远哲,吴镝,张琦..Cr2O3中反铁磁自旋波的低频拉曼光谱研究[J].物理学进展,2023,43(5):142-150,9.

基金项目

We thank Dr.Song Bao and Prof.Jin-sheng Wen for their help in the measurement of magnetic susceptibility.This work is supported by the National Key Research,Development Program of China(2020YFA0309200)and National Natural Sci-ence Foundation of China(52025012). (2020YFA0309200)

物理学进展

1000-0542

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