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多孔陶瓷负载Ce-TiO2光催化降解印染废水研究

陈伟杰 花开慧 雷鸣 王望龙

人工晶体学报2024,Vol.53Issue(1):170-180,11.
人工晶体学报2024,Vol.53Issue(1):170-180,11.

多孔陶瓷负载Ce-TiO2光催化降解印染废水研究

Photocatalytic Degradation of Dying Waste water by Porous Ceramics Supported Ce-TiO2

陈伟杰 1花开慧 2雷鸣 3王望龙3

作者信息

  • 1. 东莞理工学院生态环境与建筑工程学院,东莞 523008
  • 2. 东莞理工学院生态环境与建筑工程学院,东莞 523008||广东省城市生命线工程智慧防灾与应急技术重点实验室,东莞 523008
  • 3. 广东东实环境股份有限公司,东莞 523143
  • 折叠

摘要

Abstract

In this paper,mullite porous ceramics were prepared by dry compression molding method using construction waste as main raw material,alumina as aluminum source,aluminum fluoride as whisker catalyst,boron oxide,cerium oxide and molybdenum trioxide as sintering aids,and corn starch as pore forming additive.The effects of cerium oxide and molybdenum trioxide contents on the structure and physicochemical properties of the mullite porous ceramics were investigated,and the ceramics with the best performance were loaded with TiO2/Ce-TiO2 for photocatalytic degradation of simulated printing and dyeing wastewater.The results show that,in terms of mass fraction,when the content of cerium oxide is 4%and the content of molybdenum trioxide is 1%,the flexural strength of porous ceramics is 8.69 MPa,and the open porosity is 64.25%.Loading with 0.05 g Ce-TiO2 and mixing with 1.2 mmol/L PMS,the degradation rate of the methylene blue solution reaches 96.62%after 120 min of irradiation with LED visible light at power of 18 W and wavelength of 420~430 nm.

关键词

多孔陶瓷/莫来石晶须/可见光催化/降解/异质结/印染废水

Key words

porous ceramics/mullite whisker/visible photocatalytic/degradation/heterojunction/dying wastewater

分类

化学化工

引用本文复制引用

陈伟杰,花开慧,雷鸣,王望龙..多孔陶瓷负载Ce-TiO2光催化降解印染废水研究[J].人工晶体学报,2024,53(1):170-180,11.

基金项目

广东省普通高校创新团队项目(2019KCXTD013) (2019KCXTD013)

东莞市社会发展科技项目(20211800905302) (20211800905302)

粤澳科技创新联合资助(2022A0505020030) (2022A0505020030)

广东省基础与应用基础研究基金(19201910260000040) (19201910260000040)

广东省联合培养研究生示范基地人才培养项目(粤教研函[2021]2号,粤教研函[2023]3号) (粤教研函[2021]2号,粤教研函[2023]3号)

人工晶体学报

OA北大核心CSTPCD

1000-985X

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