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碳点/铁酸镍复合光催化剂的宽光谱芬顿降解四环素研究

袁浩 孙鑫海 李瑞广 施伟龙 郭峰

聊城大学学报(自然科学版)2024,Vol.37Issue(2):69-79,11.
聊城大学学报(自然科学版)2024,Vol.37Issue(2):69-79,11.DOI:10.19728/j.issn1672-6634.2023080004

碳点/铁酸镍复合光催化剂的宽光谱芬顿降解四环素研究

Achieving High-Efficient Broad Spectrum Driven Photo-Fenton Degradation of Tetracycline via Carbon Dots Modified NiFe2O4 Nanoparticles

袁浩 1孙鑫海 2李瑞广 1施伟龙 1郭峰2

作者信息

  • 1. 江苏科技大学材料科学与工程学院,江苏镇江 212003
  • 2. 江苏科技大学能源与动力学院,江苏镇江 212003
  • 折叠

摘要

Abstract

The synergistic reaction of photocatalysis technology and Fenton reaction is a valid strategy for the treatment of pernicious antibiotic sewage.Herein,the NiFe2O4 photocatalyst(NFO)with the function of magnetic recovery was prepared by the hydrothermal/calcination method,and further modified by load-ing carbon dots(CDs)on its surface to synthetize CDs/NFO compound,which exhibits the tetracycline(TC)photodegradation rate of 84.6%and 34.7%under visible(Vis)and near-infrared light(NIR)light irradiation,respectively.The high Vis/NIR-driven photo-Fenton catalytic degradation activity of TC over CDs/NFO photocatalysts is not only ascribed to the decomposition and regeneration process of H2O2 with cycles of Fe2+/Fe3+of NFO to generate active species,but also attributed to strong light scattering and e-lectron trapping effects of CDs.This research presents a reasonable design idea to construct a magnetic re-cyclable photo-Fenton degradation system with high-efficient activity for treatment of antibiotic wastewater.

关键词

碳点/NiFe2O4/光芬顿/可见光/近红外光/光降解

Key words

carbon dots/NiFe2O4/photo-Fenton/visible/near-infrared/photodegradation

分类

化学化工

引用本文复制引用

袁浩,孙鑫海,李瑞广,施伟龙,郭峰..碳点/铁酸镍复合光催化剂的宽光谱芬顿降解四环素研究[J].聊城大学学报(自然科学版),2024,37(2):69-79,11.

基金项目

国家自然科学基金项目(22006057)资助 (22006057)

聊城大学学报(自然科学版)

OACHSSCD

1672-6634

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