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贵州省典型铅锌矿区和贵阳市居民汞暴露以及健康风险评估

王达卫 孔林 徐晓航 韩佳良 刘杰民 仇广乐

生态学杂志2024,Vol.43Issue(3):869-877,9.
生态学杂志2024,Vol.43Issue(3):869-877,9.DOI:10.13292/j.1000-4890.202403.032

贵州省典型铅锌矿区和贵阳市居民汞暴露以及健康风险评估

Mercury exposure and health risk assessment in typical lead-zinc mining areas and Guiyang City

王达卫 1孔林 2徐晓航 3韩佳良 3刘杰民 4仇广乐3

作者信息

  • 1. 中国科学院地球化学研究所环境地球化学国家重点实验室,贵阳 550081||中国科学院大学,北京 100049
  • 2. 贵州医科大学公共卫生学院环境污染与疾病监控教育部重点实验室,贵阳 550025
  • 3. 中国科学院地球化学研究所环境地球化学国家重点实验室,贵阳 550081
  • 4. 贵州省人民医院,贵阳 550002
  • 折叠

摘要

Abstract

To assess food contamination levels of organic(MeHg)and inorganic mercury associated with mining and urban environments in Guizhou,we analyzed 503 samples from Hezhang County(lead-zinc mining area)and Guiyang.The health risk associated with dietary consumption was assessed using Monte Carlo simulations.The high-est levels of total mercury were 39 and 18 ng·g-1 in the samples from the mining area and the urban residential ar-ea,respectively.The corresponding highest measurement values for MeHg were 1.7 and 7.7 ng·g-1,respectively.The investigated foodstuffs such as rice,potatoes,chicken eggs,fish,pork did not contain significant levels of mercury contamination,with the exception of certain vegetables that frequently showed levels above the current limit standard of 10 ng·g-1.14.7%(lead/zinc mining area)and 17.7%(residential area)of vegetable samples excee-ded the limit specified in China's National Food Safety Standard(GB 2672-2017).Dietary inorganic mercury exposure was similar for food with different origins(residential area:0.031 μg·kg-1·d-1,lead-zinc mining area:0.032 μg·kg-1·d-1),while exposure to organic mercury was nearly twice greater in the urban environment(6.0 vs.3.2 ng·kg-1·d-1).In general,the average daily exposure to inorganic mercury and MeHg was lower than the provisional weekly tolerable intake(PTWI)of 4 μg·kg-1·week-1 for IHg by WHO/JECFA and the reference dose(RfD)of 0.1 μg·kg-1·d-1 for MeHg established by USEPA,respectively.Hazard index in both regions was much less than unity,suggesting no obvious non-carcinogenic health risks.

关键词

铅锌矿区/贵阳市居民区/无机汞/甲基汞/风险评估

Key words

lead-zinc mining area/Guiyang city/inorganic mercury/methylmercury/risk assessment

引用本文复制引用

王达卫,孔林,徐晓航,韩佳良,刘杰民,仇广乐..贵州省典型铅锌矿区和贵阳市居民汞暴露以及健康风险评估[J].生态学杂志,2024,43(3):869-877,9.

基金项目

贵州省科技支撑项目(黔科合支撑[2020]1Y140)、贵州高层次创新型人才项目(黔科合平台人才[2020]6016)和国家自然科学基金项目(81560773,82060850,42003065)资助. (黔科合支撑[2020]1Y140)

生态学杂志

OA北大核心CSTPCD

1000-4890

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