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碳化处理对再生微粉吸附Pb2+行为与机理的影响

王开元 萧圳坡 寇世聪 王耀城 占宝剑 邢锋

硅酸盐通报2024,Vol.43Issue(4):1420-1426,7.
硅酸盐通报2024,Vol.43Issue(4):1420-1426,7.

碳化处理对再生微粉吸附Pb2+行为与机理的影响

Effect of Carbonization Treatment on Behavior and Mechanism of Pb2+Adsorption by Recycled Concrete Fines

王开元 1萧圳坡 1寇世聪 1王耀城 1占宝剑 1邢锋1

作者信息

  • 1. 深圳大学土木与交通工程学院,深圳 518060||广东省滨海土木工程耐久性重点实验室,深圳 518060
  • 折叠

摘要

Abstract

With the development of industry,large amounts of lead-containing wastes have been discharged into the environment,causing severe pollution to water bodies.This study used carbonated recycled concrete fines(CRCF)as an adsorbent to conduct adsorption tests on lead contaminated solutions prepared with lead nitrate,and tested and analyzed its phase,microstructure,and stability of CRCF.The results indicated that CRCF possessed outstanding adsorption capacity for Pb2+,achieving a removal rate of 93.1%(mass fraction,the same below)after 24 h.The CRCF has high adsorption stability for Pb2+,with only negligible amounts of Pb2+leaching after adsorption.In the adsorption reaction,Pb2+is electrostatically adsorbed on the surface of CRCF,undergoes ion exchange with CRCF,and forms carbonate precipitation on the surface,ultimately mainly fixed in the form of carbonate in CRCF.CRCF can be used as a low-cost and efficient adsorbent for Pb2+,which can be effectively applied to the treatment of lead containing wastewater and achieve waste resource reuse.

关键词

碳化/再生混凝土微粉/吸附/Pb2+/稳定性

Key words

carbonization/recycled concrete fines/adsorption/Pb2+/stability

分类

建筑与水利

引用本文复制引用

王开元,萧圳坡,寇世聪,王耀城,占宝剑,邢锋..碳化处理对再生微粉吸附Pb2+行为与机理的影响[J].硅酸盐通报,2024,43(4):1420-1426,7.

基金项目

广东省自然科学基金面上项目(2022A1515010594) (2022A1515010594)

国家自然科学基金面上项目(52178235) (52178235)

深圳市新引进高端人才科研启动项目(827000623) (827000623)

深圳大学青年教师科研启动经费(QNJS0375) (QNJS0375)

硅酸盐通报

OA北大核心CSTPCD

1001-1625

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