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汞对低气压条件下污水处理系统脱氮性能的影响研究

高磊 戴闻 杨忠莲 李淑萍 闫刚印 孙琪 陆勇泽 朱光灿

化工学报2024,Vol.75Issue(5):2036-2046,11.
化工学报2024,Vol.75Issue(5):2036-2046,11.DOI:10.11949/0438-1157.20231393

汞对低气压条件下污水处理系统脱氮性能的影响研究

Effect of Hg on nitrogen removal performance of wastewater treatment system in low-pressure conditions

高磊 1戴闻 1杨忠莲 2李淑萍 3闫刚印 3孙琪 1陆勇泽 4朱光灿5

作者信息

  • 1. 东南大学能源与环境学院,江苏 南京 210096
  • 2. 东南大学能源与环境学院,江苏 南京 210096||西藏自治区水质安全与水环境健康重点实验室,陕西 咸阳 712082
  • 3. 西藏自治区水质安全与水环境健康重点实验室,陕西 咸阳 712082||西藏民族大学信息工程学院,陕西 咸阳 712082||西藏水污染控制与生态修复国家民委重点实验室,陕西 咸阳 712082
  • 4. 东南大学能源与环境学院,江苏 南京 210096||西藏水污染控制与生态修复国家民委重点实验室,陕西 咸阳 712082
  • 5. 东南大学能源与环境学院,江苏 南京 210096||西藏自治区水质安全与水环境健康重点实验室,陕西 咸阳 712082||西藏水污染控制与生态修复国家民委重点实验室,陕西 咸阳 712082
  • 折叠

摘要

Abstract

The presence of mercury(Hg)in wastewater treatment systems in low-pressure areas can potentially reduce the efficiency of wastewater treatment.In a laboratory-scale study using a sequencing batch reactor(SBR),the impact of Hg under low-pressure conditions on wastewater treatment systems was investigated.It was found that Hg significantly lowered the removal rate of ammonia nitrogen(NH4+-N),particularly at high concentrations.The removal rate of NH4+-N decreased from 89.73%to 38.71%with increased Hg concentrations.Hg had a detrimental effect on the nitrogen transformation process within the SBR cycle.At an influent Hg concentration of 250 μg/L,the specific ammonium oxidation rate(SAOR)and the nitrite reduction rate(SNIR)decreased by 96.74%and 96.91%,respectively,and the activities of related functional enzymes decreased by 100.00%and 97.87%,respectively.Furthermore,Hg altered the morphology and structure of the activated sludge,leading to the disintegration of the overall sludge structure and changes in surface characteristics.It also inhibited the production of extracellular polymeric substances(EPS),particularly affecting the protein content.In terms of the microbial community,the addition of Hg significantly altered the structure of the activated sludge community,especially affecting functional genera related to the nitrification process,such as Nitrosomonas and Nitrospira.Therefore,attention needs to be paid to the impact of the presence of Hg in the sewage treatment system under low-pressure conditions.

关键词

/低气压/废水/环境/微生物群落/生物过程

Key words

mercury/low-pressure/wastewater/environment/microbial community/bioprocess

分类

资源环境

引用本文复制引用

高磊,戴闻,杨忠莲,李淑萍,闫刚印,孙琪,陆勇泽,朱光灿..汞对低气压条件下污水处理系统脱氮性能的影响研究[J].化工学报,2024,75(5):2036-2046,11.

基金项目

西藏自治区科技厅自然科学基金项目(XZ202101ZR0092G) (XZ202101ZR0092G)

西藏自治区科技厅自然科学基金项目(XZ202101ZR0077G) (XZ202101ZR0077G)

国家自然科学基金项目(52160004) (52160004)

化工学报

OA北大核心CSTPCD

0438-1157

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