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烟道气CO2捕集用醇胺溶液降解研究进展OA北大核心CSTPCD

Research progress on degradation of alcoholamine solution for CO2 capture in flue gas

中文摘要英文摘要

目前在多种CO2吸收捕集技术中,醇胺法是吸收量最大、经济效益最好和研究最广泛的方法.然而,醇胺法中使用的醇胺溶液吸收剂面临的降解问题是该方法的主要缺陷.针对醇胺溶液吸收剂的降解问题,首先综述了热降解和氧化降解的产物、机理和控制研究进展,然后综述了金属离子催化降解的降解机理、规律和控制研究进展,最后对醇胺溶液吸收剂的降解问题进行了总结,并对未来的抗降解研究方向进行了展望.

At present,among the various CO2 absorption and capture technologies,the alcoholamine method is the most widely studied method with the largest amount of absorption and the best economic benefit.However,the degradation of the alcoholamine solution absorbents used in the alcoholamine method is the main defect.In view of the problem of the degradation of alcoholamine solution absorbents,the research progress on products,mechanisms and controls of thermal degradation and oxidative degradation were first reviewed.And then the research progress on mechanisms,rules and controls of metal ion catalytic degradation were reviewed.Finally,the degradation problem of alcoholamine solution absorbents was summarized,and the future research direction of anti-degradation was prospected.

陆诗建;王风;刘玲;康国俊;贡玉萍;张娟娟;刘苗苗;王宁

中国矿业大学 碳中和研究院,江苏 徐州 221116||中国矿业大学 化工学院,江苏 徐州 221116

化学工程

CO2捕集热降解氧化降解金属离子催化降解抗降解

CO2 capturethermal degradationoxidative degradationmetal ion catalytic degradationanti-degradation

《低碳化学与化工》 2024 (007)

13-22 / 10

政府间国际科技创新合作项目(2022YFE0115800);江苏省科技厅科技项目(BE2022613);江苏省煤基温室气体减排与资源化利用重点实验室创新能力建设专项(2020ZDZZ01A).

10.12434/j.issn.2097-2547.20230347

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