Blade-Coated Porous 3D Carbon Composite Electrodes Coupled with Multiscale Interfaces for Highly Sensitive All-Paper Pressure SensorsOACSTPCDEI
Flexible and wearable pressure sensors hold immense promise for health monitoring,covering disease detection and postoperative rehabilitation.Developing pressure sensors with high sensitivity,wide detection range,and cost-effectiveness is paramount.By leveraging paper for its sustainability,biocompatibility,and inherent porous structure,herein,a solution-processed all-paper resistive pressure sensor is designed with outstanding performance.A ternary composite paste,comprising a compressible 3D carbon skeleton,conductive polymer poly(3,4-ethylene dioxythiophene):poly(styrenesulfonate),and cohesive carbon nanotubes,is blade-coated on paper and naturally dried to form the porous composite electrode with hierachical micro-and nano-structured surface.Combined with screen-printed Cu electrodes in submillimeter finger widths on rough paper,this creates a multiscale hierarchical contact interface between electrodes,significantly enhancing sensitivity(1014 kPa-1)and expanding the detection range(up to 300 kPa)of as-resulted all-paper pressure sensor with low detection limit and power consumption.Its versatility ranges from subtle wrist pulses,robust finger taps,to large-area spatial force detection,highlighting its intricate submillimetermicrometer-nanometer hierarchical interface and nanometer porosity in the composite electrode.Ultimately,this all-paper resistive pressure sensor,with its superior sensing capabilities,large-scale fabrication potential,and cost-effectiveness,paves the way for next-generation wearable electronics,ushering in an era of advanced,sustainable technological solutions.
Bowen Zheng;Ruisheng Guo;Xiaoqiang Dou;Yueqing Fu;Bingjun Yang;Xuqing Liu;Feng Zhou;
State Key Laboratory of Solidification Processing,Center of Advanced Lubrication and Seal Materials,School of Materials Science and Engineering,Northwestern Polytechnical University,Xi’an 710072,People’s Republic of ChinaResearch Center of Resource Chemistry and Energy Materials,State Key Laboratory of Solid Lubrication,Lanzhou Institute of Chemical Physics,Chinese of Academy of Sciences,Lanzhou 730000,People’s Republic of ChinaState Key Laboratory of Solidification Processing,Center of Advanced Lubrication and Seal Materials,School of Materials Science and Engineering,Northwestern Polytechnical University,Xi’an 710072,People’s Republic of China Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai,Yantai 264006,People’s Republic of ChinaState Key Laboratory of Solid Lubrication,Lanzhou Institute of Chemical Physics,Chinese Academy of Sciences,Lanzhou 730000,People’s Republic of China Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai,Yantai 264006,People’s Republic of China
计算机与自动化
Micro-and nano-structuresPEDOT:PSSFlexible pressure sensorsHealth monitoringMultiscale interfaces
《Nano-Micro Letters》 2024 (012)
P.217-232 / 16
support by the Science Fund of Shandong Laboratory of Advanced Materials and Green Manufacturing at Yantai(AMGM2021A03);the"Special Lubrication and Sealing for Aerospace"Shaanxi Provincial Science and Technology Innovation Team(2024RS-CXTD-63);the Xianyang2023 Key Research and Development Plan(L2023-ZDYF-QYCX-009);the World First Class University and First Class Academic Discipline Construction Funding 2023(0604024GH0201332,0604024SH0201332).
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