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基于离散小波变换算法和Inception卷积模块一维卷积神经网络的石油类污染物红外光谱定性分析OA北大核心CSTPCD

Classification Method for Petroleum Pollutants Based on Inception-One-Dimensional Convolutional Neural Network and Infrared Spectroscopy

中文摘要英文摘要

红外光谱技术具有高效和无损等优点,在石油类污染物分类检测领域中具有重要的研究与应用价值.本研究提出了一种结合离散小波变换(DWT)算法和基于Inception卷积模块的一维卷积神经网络(Incep-tion-1D-CNN)的石油类污染物分类方法,首先使用DWT算法对原始红外光谱数据进行去噪处理,消除因实验环境、仪器误差和人工操作等因素产生的干扰信息;再通过Inception-1D-CNN模型获取多尺度的红外光谱特征信息,并基于此模型对石油类污染物进行分类预测.实验结果表明,与标准正态变换(SNV)、迭代自适应加权惩罚最小二乘法(AirPLS)和卷积平滑(S-G)预处理方法相比,DWT算法结合卷积核大小为3×1的1D-CNN模型的预测准确率为86.6%,分别提高了6.6%、6.6%和3.3%;DWT算法结合卷积核大小为5×1的1D-CNN模型的预测准确率为93.3%,分别提高了10.0%、7.0%和3.3%;DWT算法结合卷积核大小为7×1的1D-CNN模型的预测准确率为90.0%,分别提高了6.7%、10.0%和3.4%;DWT算法结合Inception-1D-CNN模型的预测准确率为100.0%,分别提高了10.0%、10.0%和3.4%.因此,结合DWT算法和Inception-1D-CNN模型能够对石油类污染物准确分类预测,为后续海面溢油污染治理提供了一定的基础.

Infrared spectroscopy technology has many advantages such as high efficiency and non-destructiveness,and has an important research and application value in the field of petroleum pollutant classification and detection.In this study,a petroleum pollutant classification method by combing the discrete wavelet transform(DWT)algorithm and a one-dimensional convolutional neural network based on the Inception module(Inception-1D-CNN)was proposed.Firstly,the DWT algorithm was used to denoise the original infrared spectral data to eliminate the interference information caused by experimental environment,instrument error and manual operation.Then,the inception-1D-CNN model was used to obtain multi-scale infrared spectroscopy feature information,and then classify the petroleum pollutants.Experimental results showed that compared with preprocessing methods such as standard normal variable(SNV),adaptive iteratively reweighted penalized least squares(AirPLS),and Savitzky-Golay smoothing(S-G),the prediction accuracy of the DWT algorithm combined with the 1D-CNN model with a convolutional kernel size of 3×1 was 86.6%,which was 6.6%,6.6%and 3.3%higher,respectively.The prediction accuracy of DWT algorithm combined with 1D-CNN model with a convolutional kernel size of 5×1 was 93.3%,which was 10.0%,7.0%and 3.3%higher,respectively.The prediction accuracy of the DWT algorithm combined with the 1D-CNN model with a convolutional kernel size of 7×1 was 90.0%,which was 6.7%,10.0%and 3.4%higher,respectively.The prediction accuracy of the DWT algorithm combined with the inception-1D-CNN model was 100.0%,which was 10.0%,10.0%and 3.4%higher,respectively.Therefore,the DWT algorithm combined with the inception-1D-CNN model could accurately classify and predict petroleum pollutants,and provided a certain basis for the subsequent treatment of oil spills on the sea surface.

孔德明;何绍炜;李心怡;赵珺瑜;宁晓东

燕山大学电气工程学院,秦皇岛 066000燕山大学信息科学与工程学院,秦皇岛 066000

红外光谱石油类污染物Inception模块卷积神经网络离散小波变换

Infrared spectrumPetroleum pollutantsInception moduleConvolution neural networkDiscrete wavelet transform

《分析化学》 2024 (009)

1287-1297 / 11

国家自然科学基金项目(No.62173289)资助. Supported by the National Natural Science Foundation of China(No.62173289).

10.19756/j.issn.0253-3820.231220

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