华侨大学学报(自然科学版)2024,Vol.45Issue(5):575-587,13.DOI:10.11830/ISSN.1000-5013.202407028
纳米结构石墨相氮化碳用于CO2催化转化的研究进展
Progress of Nanostructured Graphitic Carbon Nitride for CO2 Catalytic Conversion
摘要
Abstract
This paper comprehensively reviews the state-of-the-art advancements in graphitic carbon nitride(g-C3N4)for electrocatalytic and photocatalytic carbon dioxide reduction reaction(CO2RR).The improvement of catalytic performance by fine-tuning the key parameters of their local electronic structures,surface chemical coordination,charge transport mechanisms,and optical properties was discussed in detail.Highlighted ap-proaches encompass cutting-edge methodologies like structural optimization,defect engineering,elemental/molecular doping and heterostructure assembly,collectively offering a versatile arsenal for tailored design of g-C3N4 catalysts.The review culminates in a concise synopsis of existing challenges and future perspectives,aiming to guide the rational development of g-C3N4 as highly selective and efficient CO2 RR catalysts.关键词
石墨相氮化碳(g-C3N4)/二氧化碳还原反应(CO2RR)/催化性能/光催化/电催化/纳米结构Key words
graphitic carbon nitride(g-C3N4)/carbon dioxide reduction reaction(CO2RR)/catalytic per-formance/photocatalysis/electrocatalysis/nanostructure分类
通用工业技术引用本文复制引用
王文栋,王轶楠,饶海彬,郭芳松,詹国武..纳米结构石墨相氮化碳用于CO2催化转化的研究进展[J].华侨大学学报(自然科学版),2024,45(5):575-587,13.基金项目
国家自然科学基金资助项目(U21A20324,22278167,22322806) (U21A20324,22278167,22322806)
华侨大学科研启动项目(22BS138) (22BS138)