纳米结构石墨相氮化碳用于CO2催化转化的研究进展OACSTPCD

This paper comprehensively reviews the state-of-the-art advancements in graphitic carbon nitride(g-C3N4)for electrocatalytic and photocatalytic carbon dioxide reduction reaction(CO2RR).The improvement of catalytic performance by fine-tuning the key parameters of their local electronic structures,surface chemical coordination,charge transport mechanisms,and optical properties was discussed in detail.Highlighted ap-proaches encompass cutting-edge methodologies like structural optimization,defect engineering,elemental/molecular doping and heterostructure assembly,collectively offering a versatile arsenal for tailored design of g-C3N4 catalysts.The review culminates in a concise synopsis of existing challenges and future perspectives,aiming to guide the rational development of g-C3N4 as highly selective and efficient CO2 RR catalysts.