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纳米结构石墨相氮化碳用于CO2催化转化的研究进展

王文栋 王轶楠 饶海彬 郭芳松 詹国武

华侨大学学报(自然科学版)2024,Vol.45Issue(5):575-587,13.
华侨大学学报(自然科学版)2024,Vol.45Issue(5):575-587,13.DOI:10.11830/ISSN.1000-5013.202407028

纳米结构石墨相氮化碳用于CO2催化转化的研究进展

Progress of Nanostructured Graphitic Carbon Nitride for CO2 Catalytic Conversion

王文栋 1王轶楠 1饶海彬 1郭芳松 1詹国武1

作者信息

  • 1. 华侨大学先进碳转化技术研究院,福建厦门 362021
  • 折叠

摘要

Abstract

This paper comprehensively reviews the state-of-the-art advancements in graphitic carbon nitride(g-C3N4)for electrocatalytic and photocatalytic carbon dioxide reduction reaction(CO2RR).The improvement of catalytic performance by fine-tuning the key parameters of their local electronic structures,surface chemical coordination,charge transport mechanisms,and optical properties was discussed in detail.Highlighted ap-proaches encompass cutting-edge methodologies like structural optimization,defect engineering,elemental/molecular doping and heterostructure assembly,collectively offering a versatile arsenal for tailored design of g-C3N4 catalysts.The review culminates in a concise synopsis of existing challenges and future perspectives,aiming to guide the rational development of g-C3N4 as highly selective and efficient CO2 RR catalysts.

关键词

石墨相氮化碳(g-C3N4)/二氧化碳还原反应(CO2RR)/催化性能/光催化/电催化/纳米结构

Key words

graphitic carbon nitride(g-C3N4)/carbon dioxide reduction reaction(CO2RR)/catalytic per-formance/photocatalysis/electrocatalysis/nanostructure

分类

通用工业技术

引用本文复制引用

王文栋,王轶楠,饶海彬,郭芳松,詹国武..纳米结构石墨相氮化碳用于CO2催化转化的研究进展[J].华侨大学学报(自然科学版),2024,45(5):575-587,13.

基金项目

国家自然科学基金资助项目(U21A20324,22278167,22322806) (U21A20324,22278167,22322806)

华侨大学科研启动项目(22BS138) (22BS138)

华侨大学学报(自然科学版)

OACSTPCD

1000-5013

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