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多功能区道路灰尘中有机磷酸酯分布累积特征

金芮合 杨妤昀 邬言 杨静 刘敏

华东师范大学学报(自然科学版)Issue(6):62-73,12.
华东师范大学学报(自然科学版)Issue(6):62-73,12.DOI:10.3969/j.issn.1000-5641.2024.06.006

多功能区道路灰尘中有机磷酸酯分布累积特征

Regional-specific distribution of organophosphate esters in road dust from multiple land types

金芮合 1杨妤昀 1邬言 1杨静 1刘敏1

作者信息

  • 1. 华东师范大学地理科学学院地理信息科学教育部重点实验室,上海 200241
  • 折叠

摘要

Abstract

This study determined concentrations of more than twenty organophosphate ester(OPE)congeners in road dust samples collected from urban/suburb,agricultural,and forest regions in Hangzhou,and elucidated their spatial trends.Tris(1-chloro-2-propyl)phosphate was the predominant congener.Additionally,significant regional-specific variations in the dust-associated OPE residues were observed.High OPE concentrations were generally found in the road dust sampled from sites with high human population densities and adjacent to trunk roads,highlighting the substantial contributions of anthropogenic activities and vehicular emission to the OPE burdens.Moreover,the OPE exposure rate for the local cohorts via ingestion of and dermal contact with road dust was estimated.The estimated values of OPE exposure were at least 3-4 orders of magnitude lower than the documented reference doses,suggesting that the associated health risks to Hangzhou residents were negligible.

关键词

新污染物/有机磷酸酯/道路灰尘/空间分布/人体暴露

Key words

contaminants of emerging concern/organophosphate esters/road dust/spatial patterns/human exposure

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引用本文复制引用

金芮合,杨妤昀,邬言,杨静,刘敏..多功能区道路灰尘中有机磷酸酯分布累积特征[J].华东师范大学学报(自然科学版),2024,(6):62-73,12.

基金项目

国家自然科学基金(42230505,42107391) (42230505,42107391)

华东师范大学学报(自然科学版)

OA北大核心CSTPCD

1000-5641

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