新型炭材料(中英文)2024,Vol.39Issue(1):17-41,25.DOI:10.1016/S1872-5805(24)60833-4
碳基电催化剂缺陷工程用于CO2还原反应
Defect engineering of carbon-based electrocatalysts for the CO2 reduction reaction:A review
摘要
Abstract
Electrocatalytic carbon dioxide(CO2)reduction is an important way to achieve carbon neutrality by converting CO2 in-to high-value-added chemicals using electric energy.Carbon-based materials are widely used in various electrochemical reactions,including electrocatalytic CO2 reduction,due to their low cost and high activity.In recent years,defect engineering has attracted wide attention by constructing asymmetric defect centers in the materials,which can optimize the physicochemical properties of the mater-ial and improve its electrocatalytic activity.This review summarizes the types,methods of formation and defect characterization tech-niques of defective carbon-based materials.The advantages of defect engineering and the advantages and disadvantages of various defect formation methods and characterization techniques are also evaluated.Finally,the challenges of using defective carbon-based materials in electrocatalytic CO2 reduction are investigated and opportunities for their use are discussed.It is believed that this re-view will provide suggestions and guidance for developing defective carbon-based materials for CO2 reduction.关键词
缺陷工程/碳基材料/电催化/CO2还原Key words
Defect engineering/Carbon-based materials/Electrocatalysis/CO2 reduction分类
化学化工引用本文复制引用
卢衍堃,程白雪,战浩宇,周鹏..碳基电催化剂缺陷工程用于CO2还原反应[J].新型炭材料(中英文),2024,39(1):17-41,25.基金项目
This work was financially supported by the Nat-ural Science Foundation of Shandong Province(ZR2023QB235),Open Fund of Hubei Key Laborat-ory of Processing and Application of Catalytic Materi-als(202306404)and the Taishan Scholar Program of Shandong Province. 山东省自然科学青年基金项目(ZR2023QB235) (ZR2023QB235)
催化材料制备及应用湖北省重点实验室开放基金项目(202306404) (202306404)
山东省泰山学者工程项目. ()