新型炭材料（中英文）2024，Vol.39Issue(1)：100-130,31.DOI:10.1016/S1872-5805(24)60839-5
石墨烯基二氧化碳还原电催化材料研究进展
Graphene-based CO2 reduction electrocatalysts:A review
摘要
Abstract
The reduction of carbon dioxide(CO2)by electrochemical methods for the production of fuels and value-added chemicals is an effective strategy for overcoming the global warming problem.Due to the stable molecular structure of CO2,the design of highly selective,energy-efficient and cost-effective electrocatalysts is key.For this reason,graphene and its derivatives are competitive for CO2 electroreduction with their unique and excellent physical,mechanical and electrical properties and relatively low cost.In addition,the surface of graphene-based materials can be modified using different methods,including doping,defect engineering,production of composite structures and wrapped shapes.We first review the fundamental concepts and criteria for evaluating electrochemical CO2 reduction,as well as the catalytic principles and processes.Methods for preparing graphene-based catalysts are briefly introduced,and recent research on them is summarized according to the categories of the catalytic sites.Finally,the future development direction of CO2 electroreduction technology is discussed.关键词
石墨烯/二氧化碳还原/电催化/纳米材料/可再生能源Key words
Graphene/Carbon dioxide reduction/Electrocatalysis/Nanomaterials/Renewable energy分类
化学化工引用本文复制引用
武泽林,王聪伟,张晓祥,郭全贵,王俊英..石墨烯基二氧化碳还原电催化材料研究进展[J].新型炭材料（中英文）,2024,39(1):100-130,31.基金项目
感谢国家自然科学基金资助项目(22179138)、山西省自然科学基金(202103021224440,20210302123005)、中国科学院青年创新促进会(2020180)和山西省重大项目(20181102026). National Natural Science Foundation of China(22179138),Natural Science Foundation of Shanxi(202103021224440,20210302123005),Youth Innovation Promotion Association CAS(2020180),and Shanxi Major Project(20181102026). （22179138）
