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Al(Ⅲ)和细菌引起的含水层化学-生物复合堵塞机理研究

张一诺 阎妮

水文地质工程地质2025,Vol.52Issue(1):76-84,9.
水文地质工程地质2025,Vol.52Issue(1):76-84,9.DOI:10.16030/j.cnki.issn.1000-3665.202402012

Al(Ⅲ)和细菌引起的含水层化学-生物复合堵塞机理研究

Mechanism of chemical-biological composite clogging of aquifer caused by Al(Ⅲ)and bacteria

张一诺 1阎妮1

作者信息

  • 1. 中国海洋大学环境科学与工程学院/海洋环境科学与生态教育部重点实验室,山东 青岛 266100||中国海洋大学山东省海洋环境与地质工程重点实验室,山东 青岛 266100
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摘要

Abstract

This study investigated the chemical-biological clogging problem caused by the combined effect of aluminum trivalent[Al(Ⅲ)]and bacteria during artificial recharge processes.Laboratory-scale percolation experiments were conducted to explore the composite clogging mechanism of aquifers under the coexistence of bacteria and Al(Ⅲ)at the concentration of 0.05,0.20,and 0.60 mg/L.The results indicate that Al(Ⅲ)in the recharge water could modify the surface morphology of quartz sand and promote the chemical precipitation of aluminum-containing compounds.The formation of Si—O—Al bonds proves that the addition of Al(Ⅲ)can cause chemical clogging of the aquifer.Different concentrations of Al(Ⅲ)in the recharge water have different effects on clogging.Low Al(Ⅲ)concentrations of 0.05 and 0.20 mg/L alleviate bioclogging by inhibiting effect on bacterial activity,reducing bacterial aggregation,and overall decreasing the proportion of bacterial genera that contribute significantly to bioclogging.In contrast,high Al(Ⅲ)concentrations of 0.60 mg/L can stimulate bacteria to produce extracellular polymers(EPS),which bridge most dispersed bacteria and aggravate bioclogging.Flake deposits of aluminum-containing compounds and bacterial morphology were observed on quartz sand surface,further proving the role of Al(Ⅲ)on chemical-biological complex clogging during the recharge processes.This study provides a theoretical basis for optimizing the design and management of the recharge process by improving our understanding of the relationship between Al(Ⅲ),bacteria,and clogging effects,thus ensuring the sustainable utilization of groundwater.

关键词

Al(Ⅲ)/细菌/化学堵塞/生物堵塞/化学-生物复合堵塞/影响机制

Key words

Al(Ⅲ)/bacteria/chemical clogging/biological clogging/chemical-biological composite clogging/influence mechanism

分类

天文与地球科学

引用本文复制引用

张一诺,阎妮..Al(Ⅲ)和细菌引起的含水层化学-生物复合堵塞机理研究[J].水文地质工程地质,2025,52(1):76-84,9.

基金项目

国家自然科学基金面上项目(42277052) (42277052)

国家自然科学基金青年科学基金项目(41907161) (41907161)

水文地质工程地质

OA北大核心

1000-3665

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