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给水管网颗粒物对消毒副产物的芬顿催化去除机制

李鹏鲁 庄媛 张克峰 石宝友

环境工程学报2024,Vol.18Issue(12):3467-3474,8.
环境工程学报2024,Vol.18Issue(12):3467-3474,8.DOI:10.12030/j.cjee.202402060

给水管网颗粒物对消毒副产物的芬顿催化去除机制

Removal of DBPs by particles from drinking water distribution system through in-situ Fenton reaction

李鹏鲁 1庄媛 2张克峰 3石宝友2

作者信息

  • 1. 中国科学院生态环境研究中心,中国科学院饮用水科学与技术重点实验室,北京 100085
  • 2. 中国科学院生态环境研究中心,中国科学院饮用水科学与技术重点实验室,北京 100085||中国科学院大学,北京 100049
  • 3. 山东建筑大学市政与环境工程学院,山东济南 250101
  • 折叠

摘要

Abstract

Iron particles in drinking water distribution systems are usually regarded as pollutants that causes turbidity and color problem.This study used iron particles as a catalyst to"treat waste with waste"for in-situ removal of disinfection by-products(DBPs)in"yellow water".The results showed that the removal rates of trihalomethane and haloacetonitrile by in situ catalysis of iron particles were 51.8%and 47.6%,respectively,while the removal effect of haloacetic acid was not significant.Based on the three DBPs mentioned above,the cytotoxicity was reduced by 81.07%and the genetic toxicity was reduced by 30.46%.The two main types of crystals in the iron particles were magnetite and goethite,which are 25%and 23%,respectively,and they were key catalytic sites.The iron particles would release humic acid organic compounds into the water,hindering particle aggregation and helping to enhance catalytic activity sites.Hence,the results revealed that in-situ Fenton reaction of iron particles in the drinking water distribution systems can effectively degrade DBPs and reduce toxicity risks,providing a new approach for the in-situ Fenton reaction to weaken the toxicity risk of"yellow water".

关键词

给水管网/管垢/黄水/消毒副产物

Key words

drinking water distribution system/pipe scales/yellow water/disinfection by-products

分类

资源环境

引用本文复制引用

李鹏鲁,庄媛,张克峰,石宝友..给水管网颗粒物对消毒副产物的芬顿催化去除机制[J].环境工程学报,2024,18(12):3467-3474,8.

基金项目

国家自然科学基金资助项目(51678558) (51678558)

环境工程学报

OA北大核心CSTPCD

1673-9108

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