广东石油化工学院学报2025，Vol.35Issue(1)：66-70,5.
碘掺杂MnO2催化剂的制备及其活化过一硫酸盐降解四环素的研究
Preparation of Iodine Doped MnO2 Catalyst and Its Application for Tetracycline Degradation via Peroxymonosulfate Activation
摘要
Abstract
In this study,ammonium iodide was used as the iodine source,mixed with manganese sulfate monohydrate and ammonium persulfate in a specific ratio,and uniformly ground.By varying the calcination temperature,different iodine-doped manganese oxide catalysts(I-MnO2-1,I-MnO2-2,and I-Mn2O3)were prepared and applied to activate peroxymonosulfate(PMS)for tetracycline degradation.The results showed that the I-MnO2-1 catalyst exhibited the best performance in activating PMS for tetracycline degradation(86.9%).Within a certain range,the degradation efficiency of tetracycline increased with the dosage of the I-MnO2-1 catalyst or the concentration of PMS,with the optimal conditions being 100 mg/L of catalyst and 1 mM of PMS.This study provides a novel strategy for the rational design of highly efficient Fenton-like catalysts for wastewater treatment.关键词
二氧化锰/碘掺杂/过一硫酸盐/降解/四环素Key words
manganese dioxide/iodine doping/peroxymonosulfate/degradation/tetracycline分类
资源环境引用本文复制引用
齐岳堃,李祥,何滔,杨春平..碘掺杂MnO2催化剂的制备及其活化过一硫酸盐降解四环素的研究[J].广东石油化工学院学报,2025,35(1):66-70,5.基金项目
国家自然科学基金项目(52270064) （52270064）
广东省普通高校创新团队项目(2021KCXTD043) （2021KCXTD043）
广东省大学生"攀登计划"科技创新战略专项资金重点项目 （）
广东石油化工学院大学生创新创业训练计划项目(24A033,24B117) （24A033,24B117）
