燃料化学学报（中英文）2025，Vol.53Issue(4)：434-451,18.DOI:10.1016/S1872-5813(24)60500-1
CH4-CO2重整反应中Ni基催化剂上金属-载体相互作用研究进展
Research progress on metal-support interactions over Ni-based catalysts for CH4-CO2 reforming reaction
摘要
Abstract
With ongoing global warming and increasing energy demands,the CH4-CO2 reforming reaction(dry reforming of methane,DRM)has garnered significant attention as a promising carbon capture and utilization technology.Nickel-based catalysts are renowned for their outstanding activity and selectivity in this process.The impact of metal-support interaction(MSI),on Ni-based catalyst performance has been extensively researched and debated recently.This paper reviews the recent research progress of MSI on Ni-based catalysts and their characterization and modulation strategies in catalytic reactions.From the perspective of MSI,the effects of different carriers(metal oxides,carbon materials and molecular sieves,etc.)are introduced on the dispersion and surface structure of Ni active metal particles,and the effect of MSI on the activity and stability of DRM reactions on Ni-based catalysts is discussed in detail.Future research should focus on better understanding and controlling MSI to improve the performance and durability of nickel-based catalysts in CH4-CO2 reforming,advancing cleaner energy technologies.关键词
CO2利用/CH4-CO2重整/Ni基催化剂/金属-载体相互作用/载体Key words
CO2 utilization/CH4-CO2 reforming/Ni-based catalysts/metal-support interactions/supports分类
化学引用本文复制引用
孙凯,姜剑飞,刘紫璇,耿世奇,刘振民,杨佳茜,李莎莎..CH4-CO2重整反应中Ni基催化剂上金属-载体相互作用研究进展[J].燃料化学学报（中英文）,2025,53(4):434-451,18.基金项目
The project was supported by the Natural Science Foundation of Shanxi Province(202203021221155)and the Foundation of National Key Laboratory of High Efficiency and Low Carbon Utilization of Coal(J23-24-902). （202203021221155）
