辐射研究与辐射工艺学报2025,Vol.43Issue(2):86-97,12.DOI:10.11889/j.1000-3436.2024-0071
低温等离子体协同K2Fe4O7催化净化腈纶废水
Catalytic purification of acrylic fiber wastewater by low-temperature plasma in conjunction with K2Fe4O7
摘要
Abstract
The co-catalytic treatment of acrylic fiber wastewater using low-temperature plasma generated by a dielectric barrier discharge was studied.The solid catalyst K2Fe4O7 was synthesized by hydrothermal synthesis and characterized by X-ray diffraction and scanning electron microscopy.Wastewater samples from Sinopec Anqing Branch were used as experimental water samples,and chemical oxygen demand(COD)and turbidity were used as indices.The activity of the catalyst was first verified.Thereafter,based on a single factor experiment,a response surface method was used to optimize the test based on discharge voltage,amount of catalyst addition,and pH.The optimal response parameters were obtained as a discharge voltage of 40 kV,catalyst addition amount of 0.05 g,and pH of 2.The predicted COD degradation and turbidity removal rates of the optimal acrylic fiber wastewater were 77.43%and 91.14%,respectively.To verify the accuracy of the model,three sets of experiments were conducted under the predicted optimal experimental conditions to determine the COD degradation rate of acrylic fiber wastewater as 77.34%and turbidity removal rate as 91.11%.The accuracy of the model used in this study is relatively high.This study provides a novel approach for the purification of petrochemical wastewater.关键词
等离子体/腈纶废水/化学需氧量/降解率Key words
Plasma/Acrylic fiber wastewater/Chemical oxygen demand/Degradation rate分类
化学化工引用本文复制引用
荣俊锋,朱佳丽,赵彬彬,潘帆,张成援,陈明功..低温等离子体协同K2Fe4O7催化净化腈纶废水[J].辐射研究与辐射工艺学报,2025,43(2):86-97,12.基金项目
安徽省现代环境工程国际联合研究中心(安徽理工大学)开放基金重点项目(XDHJGC2022002),安徽理工大学专利转化培育项目(ZL201902)和国家级、省级大学生创新创业项目(202410361047、S202410361106) Supported by the Open Research Fund Program of Anhui Provincial International Joint Research Center of Modern Environmental Engineering,Anhui University of Science and Technology(XDHJGC2022002),Patent Transformation Cultivation Project of Anhui University of Science and Technology(ZL201902),and National and Provincial College Student Innovation and Entrepreneurship Projects(202410361047,S202410361106) (安徽理工大学)