应用化学2025，Vol.42Issue(7)：901-913,13.DOI:10.19894/j.issn.1000-0518.250089
三相界面调控在电催化二氧化碳还原反应中的研究进展
Research Progress on Triple-Phase Interface Engineering in Electrocatalytic CO2 Reduction Reaction
摘要
Abstract
Electrocatalytic CO2 reduction reaction(CO2RR)enables efficient synthesis of high-value chemicals and fuels,offering a promising technological pathway for mitigating atmospheric CO2 accumulation and facilitating renewable energy storage.This review presents recent advances in triple-phase interface engineering,with a particular focus on strategies to enhance CO2 diffusion and transport,as well as solutions to stability challenges in membrane electrode assemblies and gas diffusion electrode systems.Furthermore,we examine the mechanism and applicability of these strategies in optimizing catalytic activity and operational durability.Finally,we highlight the key scientific and engineering challenges that must be addressed to achieve the industrial deployment of electrocatalytic CO2RR.关键词
二氧化碳电还原反应/三相界面调控/二氧化碳传质/体系稳定性Key words
Electrochemical CO2 reduction reaction/Triple-phase interface engineering/CO2 mass transfer/System stability分类
化学化工引用本文复制引用
韩子姗,邹亢,杨雪..三相界面调控在电催化二氧化碳还原反应中的研究进展[J].应用化学,2025,42(7):901-913,13.基金项目
中石化石油化工科学研究院有限公司合同项目(No.PR20242385)资助 Supported by the SINOPEC Research Institute of Petroleum Processing Co.,Ltd.Contract Project(No.PR20242385) （No.PR20242385）
