低碳化学与化工2025，Vol.50Issue(8)：67-78,122,13.DOI:10.12434/j.issn.2097-2547.20250035
太阳能驱动天然气转化制化学品研究进展
Research progress on solar-driven conversion of natural gas to chemicals
摘要
Abstract
Under the promotion of the"carbon peaking and carbon neutrality"goals,the energy structure is accelerating its transition towards cleaner and low-carbon alternatives.Compared with coal and oil,natural gas has a lower carbon-to-hydrogen ratio and is considered one of the cleanest fossil fuels.It plays a crucial role in building a new energy system and is widely applied in hydrogen production and the synthesis of high-value carbon-containing chemicals.Although industrially mature technologies such as steam methane reforming and two-stage natural gas-to-methanol synthesis are commonly used,they generally suffer from complex processes and high energy consumption,resulting in carbon emissions that fall short of low-carbon development requirements.Solar energy,characterized by its abundance,cleanliness,low-carbon nature and renewability,offers a novel pathway for the low-carbon development of natural gas-based chemical production.On one hand,solar energy can replace traditional fossil fuels as the energy source,thereby reducing carbon emissions during production.On the other hand,solar-driven reaction pathways can help optimize reactions and simplify traditional processes.Recent research progress on both indirect and direct solar-driven natural gas conversion to chemicals was reviewed,with a particular focus on the principles and current progress on solar-driven carbon-hydrogen co-production and solar-driven chemical production from natural gas.Prospects were also presented for the design of catalytic materials and reaction systems.Simultaneously,it is pointed out that solar energy can also be used in conjunction with other new energy forms in the future,which can provide aims to provide references for the green and low-carbon transformation of natural gas-based chemical production.关键词
太阳能/天然气/氢气/高值含碳化学品Key words
solar energy/natural gas/hydrogen/high-value carbon-containing chemicals分类
能源科技引用本文复制引用
张荀,余旺,曹玥晗,郑珩,王大军,周莹..太阳能驱动天然气转化制化学品研究进展[J].低碳化学与化工,2025,50(8):67-78,122,13.基金项目
国家杰出青年科学基金(52325401) （52325401）
四川省"揭榜挂帅"项目(2023YFG0375) （2023YFG0375）
中国博士后科学基金特别资助(2024T170747). （2024T170747）
