陕西科技大学学报2025,Vol.43Issue(5):23-42,20.
等离子体催化CH4-CO2重整积碳生消机制研究进展
Research progress on carbon deposition and elimination mechanisms in plasma-catalytic reforming of CH4-CO2
摘要
Abstract
Plasma-catalytic reforming of CH4-CO2(DRM)is a green and highly efficient car-bon conversion technology capable of transforming CH4 and CO2 into high-value-added prod-ucts under mild conditions.However,the problem of catalyst carbon deposition deactivation seriously hindered the industrialization process.This review systematically examines:(1)Re-action mechanisms:The activation processes of CH4 and CO2,DRM reaction pathways,and plasma-catalyst synergistic effects;(2)Analysis of carbon deposition behavior:The types of carbon deposition,formation mechanisms,and catalyst deactivation processes;(3)Strategies for eliminating carbon deposition:plasma type,reaction condition optimization,and catalyst design.Finally,future research directions are proposed,such as developing highly carbon-re-sistant catalysts and optimizing reactor configurations,providing theoretical insights for un-derstanding carbon deposition in plasma-catalytic DRM processes.关键词
等离子体/CH4-CO2重整/积碳/形成和消除Key words
plasma/CH4-CO2 reforming/carbon deposition/formation and elimination分类
化学化工引用本文复制引用
畅选辰,常甜,胡锦超,尚倩,史珂凡..等离子体催化CH4-CO2重整积碳生消机制研究进展[J].陕西科技大学学报,2025,43(5):23-42,20.基金项目
国家自然科学基金项目(22208204) (22208204)
中国博士后科学基金项目(2022M722015) (2022M722015)
陕西省自然科学基础研究计划项目(2022JQ-101) (2022JQ-101)
陕西省创新能力支撑计划项目(2024WZ-YBXM-18) (2024WZ-YBXM-18)
陕西省博士后科研项目(2023) (2023)
西安交通大学电力设备电气绝缘国家重点实验室科研项目(EIPE23213) (EIPE23213)
陕西科技大学环境科学与工程学院研究生科研创新基金项目(2025) (2025)