天津工业大学学报2026，Vol.45Issue(2)：67-76,10.DOI:10.3969/j.issn.1671-024x.2026.02.009
基于单原子催化PMS产生单线态氧在水净化中的研究进展
Research progress on single-atom catalysis for peroxymonosulfate(PMS)activation to generate singlet oxygen in water purification
摘要
Abstract
Singlet oxygen(1O2)is a kind of reactive oxygen species with mild oxidative potential,which is generated by peroxymonosulfate(PMS)activation over single-atom catalysts(SACs),showcasing excellent reactivity and selectivity toward electron-rich pollutants in water.This paper reviews the research progress of 1O2 production by SACs/PMS systems toward water pollution abatement.The essential roles of 1O2 in SACs are emphasized by summarizing the active centers of SACs,the reaction pathways of 1O2,as well as the pollution abatement efficiencies.Moreover,the identification methods of 1O2 and their existing problems are analyzed,while the future directions are outlooked.This review aims to provide guidance for the development of green and efficient SACs to exert the selective oxidation advantages of 1O2.关键词
单线态氧/单原子催化/过氧单硫酸盐/水污染控制/作用机理Key words
singlet oxygen/single-atom catalysis/peroxymonosulfate(PMS)/water pollution control/reaction mechanism分类
化学化工引用本文复制引用
王骏,毕思梦,褚梦旭,林雅洁,张阳,谭小耀..基于单原子催化PMS产生单线态氧在水净化中的研究进展[J].天津工业大学学报,2026,45(2):67-76,10.基金项目
国家自然科学基金项目(22376158,21906117) （22376158,21906117）
河北省自然科学基金项目(B2023110008) （B2023110008）
