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On-surface synthesis and interfacial charge redistribution of open-shell[3]triangulene-fused porphyrins on Au(111)

Miguel Martínez García Roman Fasel Giovanni Bottari Feifei Xiang Andres Ortega-Guerrero Manish Kumar Nicolò Bassi Carlo A.Pignedoli Pascal Ruffieux Tomas Torres Pavel Jelínek

国家科学评论（英文版）Issue(7)：38-47,10.

国家科学评论（英文版）Issue(7)：38-47,10.DOI:10.1093/nsr/nwag155

On-surface synthesis and interfacial charge redistribution of open-shell[3]triangulene-fused porphyrins on Au(111)

Miguel Martínez García ¹Roman Fasel ²Giovanni Bottari ³Feifei Xiang ⁴Andres Ortega-Guerrero ⁵Manish Kumar ⁶Nicolò Bassi ⁵Carlo A.Pignedoli ⁵Pascal Ruffieux ⁵Tomas Torres ³Pavel Jelínek⁶

作者信息

1. Departamento de Química Orgánica,Universidad Autónoma de Madrid,Campus de Cantoblanco,Madrid 28049,Spain||IMDEA Nanociencia,Campus de Cantoblanco,Madrid 28049,Spain
2. nanotech@surfaces Laboratory,Empa-Swiss Federal Laboratories for Materials Science and Technology,Dübendorf 8600,Switzerland||Department of Chemistry,Biochemistry and Pharmaceutical Sciences,University of Bern,Bern 3012,Switzerland
3. Departamento de Química Orgánica,Universidad Autónoma de Madrid,Campus de Cantoblanco,Madrid 28049,Spain||IMDEA Nanociencia,Campus de Cantoblanco,Madrid 28049,Spain||Institute for Advanced Research in Chemical Sciences(IAdChem),Universidad Autońoma de Madrid,Madrid 28049,Spain
4. nanotech@surfaces Laboratory,Empa-Swiss Federal Laboratories for Materials Science and Technology,Dübendorf 8600,Switzerland||School of Advanced Manufacturing Engineering,Nanjing University,Suzhou 215163,China
5. nanotech@surfaces Laboratory,Empa-Swiss Federal Laboratories for Materials Science and Technology,Dübendorf 8600,Switzerland
6. Institute of Physics,Czech Academy of Sciences,Prague 16200,Czech Republic
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摘要

关键词

graphene/magnetism/many-body states/scanning tunneling microscopy/charge transfer

Key words

graphene/magnetism/many-body states/scanning tunneling microscopy/charge transfer

引用本文复制引用

Miguel Martínez García,Roman Fasel,Giovanni Bottari,Feifei Xiang,Andres Ortega-Guerrero,Manish Kumar,Nicolò Bassi,Carlo A.Pignedoli,Pascal Ruffieux,Tomas Torres,Pavel Jelínek..On-surface synthesis and interfacial charge redistribution of open-shell[3]triangulene-fused porphyrins on Au(111)[J].国家科学评论（英文版）,2026,(7):38-47,10.

基金项目

G.B.and T.T.acknowledge financial support from the Spanish MICINN/AEI/10.13039/501100011033(PID2020-116490GB-I00,PID2023-151167NB-I00 and TED2021-131255B-C43),the Comunidad de Madrid and the Spanish State through the Recovery,Transformation and Resilience Plan('Materiales Disruptivos Bidimensionales(2D)'(MAD2D-CM)(UAM1)-MRR Materiales Avanzados),and the Euro-pean Union through the Next Generation EU funds.IMDEA Nanociencia acknowledges support from the'SeveroOchoa'Programme for Centres of Excellence in R&D(MINECO,SEV-2016-0686).T.T.also acknowledges the Alexander von Humboldt Foundation(Germany)for the A.v.Humboldt-J.C.Mutis Research Award 2023(Ref 3.3-1231125-ESP-GSA).R.F.acknowledges financial support from the Swiss National Science Foundation(212875)and the Werner Siemens Foun-dation(CarboQuant).C.A.P.and A.O.-G.acknowledge the Swiss Supercomputing Center(CSCS)for computing re-sources(lp83)and the NCCR MARVEL,a National Centre of Competence in Research funded by the Swiss National Science Foundation(205602).F.X.thanks the Deutsche Forschungs-gemeinschaft(DFG)for a Walter Benjamin Fellowship(452269487)and the SNSF for a Postdoctoral Fellowship(210093).P.J.and M.K.acknowledge the support from GACR 25-17866X,the CzechNanoLab Research Infrastructure supported by MEYS CR(LM2023051),and the financial support from the TERAFIT project(CZ.02.01.01/00/22_008/0004594). （PID2020-116490GB-I00,PID2023-151167NB-I00 and TED2021-131255B-C43）

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