土壤学报2026，Vol.63Issue(2)：435-448,14.DOI:10.11766/trxb202507040328
某历史不规范填埋场及周边农田土壤微塑料污染特征与生态风险评估
Microplastic Pollution Characteristics and Ecological Risk Assessment in Soils of a Historical Non-Sanitary Landfill and Adjacent Farmland
摘要
Abstract
[Objective]Historically non-sanitary landfills continuously release microplastics(MPs)into adjacent soils due to the absence of impermeable lining systems,thereby exacerbating ecological risks at the site and in surrounding environments.This study aims to investigate the distribution characteristics and ecological risks of MPs in a historically non-sanitary landfill and adjacent farmland soils in Jiashan County,Zhejiang Province,East China.The research aims to identify key pollution sources and evaluate the efficacy of multi-method risk assessment frameworks for informing targeted pollution control strategies.[Method]For landfill sites and surrounding farmland topsoil,the distribution characteristics and ecological risks of microplastic pollution were revealed through the combined application of micro-Fourier transform infrared spectroscopy(μ-FTIR),the Pollution Load Index(PLI),Risk Characterization Ratio(RCR),the Multi-characteristics Potential Ecological Risk Index(MPERI),and Monte Carlo simulation.[Result](1)Landfill soils exhibited significantly higher MPs abundance(7 425.5-21 306.5 items/kg)than farmland soils(199.5-2,868.5 items/kg).Polyethylene terephthalate(PET)and polyethylene(PE)were the main MP types in both sites(＞70％of total MPs).Small-sized MPs(＜1 mm)accounted for 70.9％in landfill soil and 66.3％in farmland soil,while transparent MPs comprised 71.8％and 53.1％in landfill and farmland soil,respectively.The landfill was identified as a potential source of farmland MPs.(2)Multi-model risk assessment revealed that PLI classified the landfill as medium-to-high risk and farmland as low-to-medium risk,whereas RCR and MPERI indicated low-to-medium risk for both.Risk escalated significantly at sites containing acrylonitrile resin(PAN).(3)Monte Carlo simulations demonstrated that farmland had a higher probability of low PLI risk than the landfill.Nevertheless,both RCR and MPERI might underestimate ecological risks in the landfill.Sensitivity analysis identified MPs polymer type as the paramount parameter influencing risk outcomes.[Conclusion]The landfill acts as a critical source of MPs contamination in adjacent agricultural soils.Discrepancies in risk outcomes across models highlight the necessity of integrating multi-method assessments with probabilistic approaches(e.g.,Monte Carlo)to quantify uncertainties.Polymer type is a decisive factor in ecological risk,necessitating prioritized controls for PAN-containing MPs.This empirical-modeling framework provides a scientific basis for hierarchical management of MPs pollution in non-sanitary landfills and surrounding environments,promoting the application of probabilistic risk models in contaminated sites.关键词
历史不规范填埋场/土壤污染/微塑料/生态风险评估Key words
Historical non-sanitary landfills/Soil contamination/Microplastics/Ecosystem risk assessment分类
资源环境引用本文复制引用
张鹏,彭程,陈小艺,刘惠,隋倩,张卫..某历史不规范填埋场及周边农田土壤微塑料污染特征与生态风险评估[J].土壤学报,2026,63(2):435-448,14.基金项目
国家重点研发计划项目(2023YFC3711600)资助Supported by the National Key Research and Development Program of China(No.2023YFC3711600) （2023YFC3711600）
