高校化学工程学报2026,Vol.40Issue(3):379-395,17.DOI:10.3969/j.issn.1003-9015.2025.00.069
基于气液多相反应过程强化的CO2捕集研究进展
Research progress on CO2 capture based on intensification of gas-liquid multiphase reaction processes
摘要
Abstract
The development of efficient carbon capture technologies is a key pathway to achieve the"dual carbon"goals.Chemical absorption,characterized by high mass transfer efficiency,rapid reaction kinetics,and mature process engineering,has established itself as a prominent technical solution for post-combustion carbon capture.In recent years,significant advancements have been attained in absorbent development,bubble behavior modulation,mass transfer mechanism elucidation,and reactor configuration design.Nevertheless,substantial challenges persist in energy consumption control,interfacial stability maintenance,and process intensification pathways.This review critically synthesizes the state-of-the-art progress in typical absorbent systems and their synergistic mechanisms,bubble dispersion characteristics,multiphase interfacial mass transfer behaviors,reactor optimization methodologies,and the impacts of key operating parameters on system performance.The article also evaluates the synergistic regulation potential of external physical fields,including electric and magnetic fields.Future research directions are proposed from the perspectives of multiscale modeling,phase dispersion intensification,and functional material design,with the aim of providing theoretical foundations and technical references for the construction of high-efficiency,low-energy-consumption,and environmentally benign carbon capture systems.关键词
鼓泡反应器/二氧化碳捕集/气泡/化学吸收剂/传质效率/多相反应Key words
bubble column reactor/CO2 capture/bubble/chemical absorbent/mass transfer efficiency/multiphase reaction分类
能源科技引用本文复制引用
张亚栋,张伟,詹水清,王家乐,王军锋..基于气液多相反应过程强化的CO2捕集研究进展[J].高校化学工程学报,2026,40(3):379-395,17.基金项目
国家自然科学基金项目(52206201,52476154). (52206201,52476154)