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低浓度CO2条件40℃环境对水泥胶砂早期碳化与水化反应进程影响研究

胡庆浩 李绍纯 陈旭 张书畅

硅酸盐通报2026,Vol.45Issue(6):1892-1902,11.
硅酸盐通报2026,Vol.45Issue(6):1892-1902,11.DOI:10.16552/j.cnki.issn1001-1625.2025.1148

低浓度CO2条件40℃环境对水泥胶砂早期碳化与水化反应进程影响研究

Influence of Low-Concentration CO2 Environment at 40℃on Early Carbonation and Hydration Reaction Process of Cement Mortar

胡庆浩 1李绍纯 1陈旭 2张书畅1

作者信息

  • 1. 青岛理工大学土木工程学院,青岛 266520
  • 2. 新疆大学建筑工程学院,乌鲁木齐 830047
  • 折叠

摘要

Abstract

In response to the low-carbon development strategy for building materials,this study explores the optimization path for early-age performance of cement-based materials under low-concentration CO2 conditions.Cement mortars were subjected to CO2 curing at 3%(volume fraction)concentration and 40℃for 2,6,and 12 h to investigate the effects of the carbonation-hydration synergy on mechanical properties,microstructure evolution.The results show that the comprehensive performance of cement-based materials is optimal after 6 h of carbonation,with a 28 d compressive strength of 58.6 MPa—approximately 15.1%higher than that of the purely hydrated sample.At this stage,the amount and crystallinity of CaCO3 reach their maximum,and the proportion of calcite increases significantly.Mercury intrusion porosimetry results reveal that 6 h carbonation effectively refines the pore structure of the specimen surface layer,reducing porosity to 21.8% and enhancing compactness and stability of the material.However,extending the carbonation time causes deterioration of the surface pore structure,leading to reduce strength due to over-carbonation.

关键词

水泥基材料/低浓度CO2/早期碳化/温度调控/微观结构演化

Key words

cement-based material/low-concentration CO2/early-age carbonation/temperature regulation/microstructural evolution

分类

建筑与水利

引用本文复制引用

胡庆浩,李绍纯,陈旭,张书畅..低浓度CO2条件40℃环境对水泥胶砂早期碳化与水化反应进程影响研究[J].硅酸盐通报,2026,45(6):1892-1902,11.

基金项目

国家自然科学基金(52479125) (52479125)

丝绸之路经济带创新驱动发展试验区、乌昌石国家自主创新示范区科技发展计划(2022LQ03010) (2022LQ03010)

硅酸盐通报

1001-1625

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