Deformable Catalytic Material Derived from Mechanical Flexibility for Hydrogen Evolution ReactionOACSTPCD
Deformable Catalytic Material Derived from Mechanical Flexibility for Hydrogen Evolution Reaction
Deformable catalytic material with excellent flexible structure is a new type of catalyst that has been applied in various chemical reactions,especially elec-trocatalytic hydrogen evolution reaction(HER).In recent years,deformable catalysts for HER have made great progress and would become a research hotspot.The cata-lytic activities of deformable catalysts could be adjustable by the strain engineering and surface reconfiguration.The surface curvature of flexible catalytic materials is closely related to the electrocatalytic HER properties.Here,firstly,we systematically summarized self-adaptive catalytic performance of deformable catalysts and vari-ous micro-nanostructures evolution in catalytic HER process.Secondly,a series of strategies to design highly active catalysts based on the mechanical flexibility of low-dimensional nanomaterials were summarized.Last but not least,we presented the challenges and prospects of the study of flexible and deformable micro-nanostruc-tures of electrocatalysts,which would further deepen the understanding of catalytic mechanisms of deformable HER catalyst.
Fengshun Wang;Longlu Wang;Lingbin Xie;Ning Sun;Ting Zhi;Mengyang Zhang;Yang Liu;Zhongzhong Luo;Lanhua Yi;Qiang Zhao
College of Electronic and Optical Engineering & College of Flexible Electronics(Future Technology),Nanjing University of Posts &Telecommunications(NJUPT),9 Wenyuan,Nanjing 210023,People's Republic of ChinaKey Laboratory of Environmentally Friendly Chemistry and Applications of Ministry of Education,School of Chemistry,Xiangtan University,Xiangtan 411105,People's Republic of ChinaCollege of Electronic and Optical Engineering & College of Flexible Electronics(Future Technology),Nanjing University of Posts &Telecommunications(NJUPT),9 Wenyuan,Nanjing 210023,People's Republic of China||State Key Laboratory of Organic Electronics and Information Displays & Jiangsu Key Laboratory for Biosensors,Institute of Advanced Materials(IAM)& Institute of Flexible Electronics(Future Technology),Nanjing University of Posts & Telecommunications,9 Wenyuan,Nanjing 210023,People's Republic of China
Deformable catalytic materialMicro-nanostructures evolutionMechanical flexibilityHydrogen evolution reaction
《纳微快报（英文）》 2024 (002)
287-311 / 25
This work was financially supported by the National Natural Science Foundation of China(Nos.51902101 and 21875203),the Natural Science Foundation of Hunan Province(Nos.2021JJ40044 and 2023JJ50287),Natural Science Foundation of Jiangsu Province(No.BK20201381).Open access funding provided by Shanghai Jiao Tong University.
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