炭载单原子催化剂在电化学反应中的应用进展OA北大核心CSTPCD
A review of carbon-supported single-atom catalysts for electrochemical reactions
本文全面综述了用于电化学反应的炭载单原子催化剂(SAC)的最新进展.首先简要介绍了炭载单原子催化剂的发展和优势,然后详细总结了各种炭载单原子催化剂的合成策略,包括气相传输、高温热解和湿化学方法.随后,回顾了炭载SAC的先进表征技术,总结了炭载SAC在氧气还原反应、二氧化碳还原反应、氮气还原反应、氢气进化反应和氧气进化反应等不同领域的应用.特别强调了提高炭载SACs电催化性能的改性策略.最后,讨论了利用炭载SAC进行电化学反应的前景和挑战.
Recent advances in the use of carbon-supported single-atom catalysts(SACs)for electrochemical reactions are com-prehensively reviewed.The development and advantages of carbon-supported SACs are briefly introduced,followed by a detailed summary of the synthesis strategies used,including vapor phase transport,high temperature pyrolysis and wet chemical methods.Ad-vanced characterization techniques for carbon-supported SACs are also reviewed.The use of carbon-supported SACs in different fields,such as the oxygen reduction reaction,carbon dioxide reduction reaction,nitrogen reduction reaction,hydrogen evolution re-action,and oxygen evolution reaction are summarized.Special emphasis is given to the modification strategies used to enable car-bon-supported SACs to have an excellent electrocatalytic performance.Finally,the prospects and challenges associated with using carbon-supported SACs for electrochemical reactions are discussed.
王翊丞;张亚婷;马晓博;Ayeza;王晨旭;李阳;杨成龙;王哲帆;汪超;胡超
西安科技大学 化学与化工学院,陕西 西安,710054西安交通大学 化学工程与技术学院,陕西 西安,710049||清华大学深圳国际研究生院,广东 深圳,518055西安交通大学 化学工程与技术学院,陕西 西安,710049西安热工研究院有限公司,陕西 西安,710054
单原子催化剂炭电化学反应合成改性
Single-atom catalystsCarbonElectrochemical reactionsSynthesisModification
《新型炭材料（中英文）》 2024 (003)
407-438 / 32
This work was supported by the National Natur-al Science Foundation of China(51702254,52102051),the Fundamental Research Funds for the Central Universities(xhj032021011-05),Shaanxi Pro-vincial Innovation Capacity Support Programme Project(2019-TD-021),and Science and Technology Project of China Huaneng Group Co.,Ltd.(HNKJ21-H32). 国家自然科学基金(51702254、52102051);中央高校基本科研业务费(xhj032021011-05);陕西省创新能力支撑计划项目(2019-TD-021);中国华能集团有限公司科技项目(HNKJ21-H32).
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