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固态锂金属电池正极/电解质界面研究进展OA北大核心CSTPCD

Research progress on cathode/electrolyte interface optimization of solid-state lithium metal batteries

中文摘要英文摘要

固态锂金属电池以其突出的安全性与高理论比容量成为目前最具发展前景的锂电池技术.在构建高比能固态锂电池体系时,如何较好地解决正极与固体电解质之间的界面问题以及二者之间的兼容性,是高安全性和高比能量固态锂电池技术的痛点之一.通过对固体电解质膜机械特性改性、正极/电解质界面特性改性及其一体化制备技术、界面理论计算等介绍,总结综述了如优化固态电解质与正极材料的物理接触、加强正极/电解质渗透性、改善界面兼容性和正极/电解质固体界面相构建等正极/电解质界面改性技术进展情况,并对固态锂金属电池界面改性技术的发展趋势做了展望.

Solid-state lithium metal battery has become the most promising lithium battery technol-ogy for its outstanding safety and high theoretical specific capacity. For building a system with high specific energy density,the main obstacle is the interfacial issues and the compatibility between cath-ode and solid electrolyte. Through the introduction of modification strategies on film mechanical property,cathode/electrolyte interface properties and its integrated preparation technology,and theo-retical calculation,etc,the progress of cathode/electrolyte interfacial modification techniques such as physical contact optimization,cathode/electrolyte permeability enhancement,interface compatibility improvement and cathode electrolyte interphase construction were reviewed. The development trend of interface modification technology for solid-state lithium metal batteries was also prospected.

王冠华;张宇航;刘峰;李德平;吴禹翰

沈阳工业大学环境与化学工程学院,辽宁沈阳110870沈阳工业大学材料科学与工程学院,辽宁沈阳110870哈尔滨工业大学(深圳)材料科学与工程学院,广东深圳518055沈阳工业大学环境与化学工程学院,辽宁沈阳110870||南开大学先进能源材料化学教育部重点实验室,天津300071

动力与电气工程

固态锂金属电池正极/电解质界面界面工程

solid-state lithium metal batterycathode/electrolyte interfaceinterface engineering

《电源技术》 2024 (008)

1420-1431 / 12

辽宁省教育厅基本科研项目(JYTQN2023285);国家自然科学基金(21571132);功能无机材料化学教育部重点实验室开放课题;辽宁省自然科学基金联合基金(2023-BSBA-250,2023-BSBA-260);沈阳工业大学青年教师科研能力培育基金(QNPY202209-4)

10.3969/j.issn.1002-087X.2024.08.003

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